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High-Entropy-Alloy Nanoparticles with Enhanced Interband Transitions for Efficient Photothermal Conversion
Angewandte Chemie International Edition ( IF 16.1 ) Pub Date : 2021-10-04 , DOI: 10.1002/anie.202112520
Yixing Li 1 , Yijun Liao 1 , Jian Zhang 2 , Enhui Huang 3 , Lianze Ji 1, 2 , Zhengyu Zhang 1 , Rongzhi Zhao 1, 2 , Zhimin Zhang 1 , Bo Yang 1 , Yanhui Zhang 1 , Bo Xu 3 , Gaowu Qin 1 , Xuefeng Zhang 1, 2
Affiliation  

A strategy toward the optimization of photothermal conversion materials with broad optical absorption and high conversion efficiency via the d-d interband transitions is demonstrated. The high-entropy-alloy nanoparticles could realize an excellent solar harvesting performance especially compositing with up to seven 3d elements in a single phase, ascribing to the fully filled energy regions below and above the Fermi level.
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中文翻译:

具有增强的带间跃迁的高熵合金纳米粒子可实现高效的光热转换

展示了一种通过 dd 带间跃迁优化具有宽光吸收和高转换效率的光热转换材料的策略。高熵合金纳米粒子可以实现出色的太阳能收集性能,尤其是在单相中与多达七个 3d 元素复合,这归因于费米能级下方和上方的完全填充的能量区域。
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更新日期:2021-12-13
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