Metal–Organic Frameworks Derived Functional Materials for Electrochemical Energy Storage and Conversion: A Mini Review,Nano Letters

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Metal–Organic Frameworks Derived Functional Materials for Electrochemical Energy Storage and Conversion: A Mini Review
Nano Letters ( IF 9.6 ) Pub Date : 2021-02-10 , DOI: 10.1021/acs.nanolett.0c04898
Xue Feng Lu ₁ , Yongjin Fang ₁ , Deyan Luan ₁ , Xiong Wen David Lou ₁

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With many apparent advantages including high surface area, tunable pore sizes and topologies, and diverse periodic organic–inorganic ingredients, metal–organic frameworks (MOFs) have been identified as versatile precursors or sacrificial templates for preparing functional materials as advanced electrodes or high-efficiency catalysts for electrochemical energy storage and conversion (EESC). In this Mini Review, we first briefly summarize the material design strategies to show the rich possibilities of the chemical compositions and physical structures of MOFs derivatives. We next highlight the latest advances focusing on the composition/structure/performance relationship and discuss their practical applications in various EESC systems, such as supercapacitors, rechargeable batteries, fuel cells, water electrolyzers, and carbon dioxide/nitrogen reduction reactions. Finally, we provide some of our own insights into the major challenges and prospective solutions of MOF-derived functional materials for EESC, hoping to shed some light on the future development of this highly exciting field.

中文翻译：

金属-有机框架衍生的用于电化学能量存储和转换的功能材料：概述

具有许多明显的优势，包括高表面积，可调节的孔径和拓扑结构以及多种周期性的有机-无机成分，金属-有机骨架（MOF）被确定为通用的前体或牺牲模板，可用于将功能材料制备为高级电极或高效材料用于电化学能量存储和转化的催化剂（EESC）。在本迷你评论中，我们首先简要概述材料设计策略，以显示MOF衍生物的化学组成和物理结构的丰富可能性。接下来，我们重点介绍成分/结构/性能关系的最新进展，并讨论它们在各种EESC系统中的实际应用，例如超级电容器，可充电电池，燃料电池，水电解槽，和二氧化碳/氮气还原反应。最后，我们提供了自己的见解，以了解MOF衍生的功能材料对EESC的主要挑战和预期解决方案，以期为这一激动人心的领域的未来发展提供一些启示。

更新日期：2021-02-24

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