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Recent Progress of Transition Metal Phosphides for Photocatalytic Hydrogen Evolution
ChemSusChem ( IF 7.5 ) Pub Date : 2020-11-20 , DOI: 10.1002/cssc.202002454 Long‐fei Hong 1 , Rui‐tang Guo 1, 2, 3 , Ye Yuan 1 , Xiang‐yin Ji 1 , Zhi‐dong Lin 1 , Zheng‐sheng Li 1 , Wei‐guo Pan 1, 3
ChemSusChem ( IF 7.5 ) Pub Date : 2020-11-20 , DOI: 10.1002/cssc.202002454 Long‐fei Hong 1 , Rui‐tang Guo 1, 2, 3 , Ye Yuan 1 , Xiang‐yin Ji 1 , Zhi‐dong Lin 1 , Zheng‐sheng Li 1 , Wei‐guo Pan 1, 3
Affiliation
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Photocatalytic hydrogen evolution can effectively alleviate the troublesome global energy crisis by converting solar energy into the chemical energy of hydrogen. In order to realize efficient hydrogen generation, a variety of semiconductor materials have been extensively investigated, including TiO2, CdS, g‐C3N4, metal‐organic frameworks (MOFs), and others. In recent years, to achieve higher photocatalytic performance and reach the level of large‐scale industrial applications, photocatalysts decorated with transition metal phosphides (TMPs) have shone brightly because of their low cost, stable physical and chemical properties, and substitution for precious metals of TMPs. This Review highlights the preparation methods and properties associated with photocatalysis of TMPs. Moreover, the H2 generation efficiency of photocatalysts loaded with TMPs and the roles of TMPs in catalytic systems are also studied systematically. Apart from being co‐catalysts, several TMPs can also serve as host catalysts to boost the activity of photocatalytic composites. Finally, the development prospects and challenges of TMPs are put forward, which is valuable for future researchers to expand the application of TMPs in photocatalytic directions and to develop more active photocatalytic systems.
中文翻译：
过渡金属磷化物光催化制氢的新进展
通过将太阳能转化为氢的化学能，光催化氢的释放可以有效缓解麻烦的全球能源危机。为了实现高效的制氢，已广泛研究了多种半导体材料，包括TiO 2，CdS，g‐C 3 N 4。，金属有机框架（MOF）等。近年来，为实现更高的光催化性能并达到大规模工业应用水平，用过渡金属磷化物（TMP）装饰的光催化剂因其成本低，稳定的物理和化学性质以及可替代的贵金属而光彩照人。 TMP。这篇综述重点介绍了与TMPs光催化相关的制备方法和性质。而且，H 2还系统地研究了载有TMP的光催化剂的产生效率以及TMP在催化体系中的作用。除了作为助催化剂外，几种TMP还可以用作主体催化剂来增强光催化复合材料的活性。最后，提出了TMPs的发展前景和挑战，这对于未来的研究者扩展TMPs在光催化方向上的应用以及开发更具活性的光催化体系具有重要的参考价值。
更新日期：2021-01-25
中文翻译：
过渡金属磷化物光催化制氢的新进展
通过将太阳能转化为氢的化学能，光催化氢的释放可以有效缓解麻烦的全球能源危机。为了实现高效的制氢，已广泛研究了多种半导体材料，包括TiO 2，CdS，g‐C 3 N 4。，金属有机框架（MOF）等。近年来，为实现更高的光催化性能并达到大规模工业应用水平，用过渡金属磷化物（TMP）装饰的光催化剂因其成本低，稳定的物理和化学性质以及可替代的贵金属而光彩照人。 TMP。这篇综述重点介绍了与TMPs光催化相关的制备方法和性质。而且，H 2还系统地研究了载有TMP的光催化剂的产生效率以及TMP在催化体系中的作用。除了作为助催化剂外，几种TMP还可以用作主体催化剂来增强光催化复合材料的活性。最后，提出了TMPs的发展前景和挑战，这对于未来的研究者扩展TMPs在光催化方向上的应用以及开发更具活性的光催化体系具有重要的参考价值。
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