MXene has been considered as a promising electrode materials for energy storage devices. This work reports using an electrophoresis effect to efficiently deposit Ti₃C₂T_x/rGO composite on flexible substrates, which are subsequently used as the electrodes of all-solid-state supercapacitors. The electrophoresis deposition does not require a binder in the fabrication of the Ti₃C₂T_x/rGO electrodes. The structures and properties of the MXene/graphene electrode materials are characterized using Zeta potential, scanning electronic microscope, X-ray powder diffraction, Fourier-transform infrared and X-ray photoelectron spectroscopy. The performance of the all-solid-state flexible supercapacitors are evaluated using cyclic voltammetry, galvanostatic charge/discharge, electrochemical impedance spectroscopy, and cycle life tests. The devices show high areal specific capacitance of ~12 mF cm⁻², small resistance, and excellent cycling stability at different current densities for over 4,000 cycles. Moreover, the all-solid-state flexible supercapacitors exhibit superior mechanical flexibility under different deformations.

MXene被认为是用于能量存储设备的有前途的电极材料。这项工作报道了利用电泳效应在柔性基板上有效沉积Ti ₃ C ₂ T _x / rGO复合材料，然后将其用作全固态超级电容器的电极。电泳沉积在Ti ₃ C ₂ T _x的制造中不需要粘合剂/ rGO电极。利用Zeta电位，扫描电子显微镜，X射线粉末衍射，傅立叶变换红外光谱和X射线光电子能谱对MXene /石墨烯电极材料的结构和性能进行表征。使用循环伏安法，恒电流充/放电，电化学阻抗谱和循环寿命测试来评估全固态柔性超级电容器的性能。这些器件在超过4000个循环中显示出约12 mF cm ^-2的高面积比电容，小的电阻以及在不同电流密度下的出色循环稳定性。而且，全固态柔性超级电容器在不同变形下表现出优异的机械柔性。