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Spinel-structure catalyst catalyzing CO2 hydrogenation to full spectrum alkenes with an ultra-high yield.
Chemical Communications ( IF 4.3 ) Pub Date : 2020-07-08 , DOI: 10.1039/d0cc03426f Lisheng Guo 1 , Jie Li , Yu Cui , Rungtiwa Kosol , Yan Zeng , Guangbo Liu , Jinhu Wu , Tiansheng Zhao , Guohui Yang , Lishu Shao , Peng Zhan , Jienan Chen , Noritatsu Tsubaki
Chemical Communications ( IF 4.3 ) Pub Date : 2020-07-08 , DOI: 10.1039/d0cc03426f Lisheng Guo 1 , Jie Li , Yu Cui , Rungtiwa Kosol , Yan Zeng , Guangbo Liu , Jinhu Wu , Tiansheng Zhao , Guohui Yang , Lishu Shao , Peng Zhan , Jienan Chen , Noritatsu Tsubaki
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Spinel-like ZnFe2O4 is tailor-made synthesized for catalyzing CO2 hydrogenation, achieving an ultra-high yield (1858.1 g kgcat−1 h−1) of full spectrum alkenes in a three-stage reactor system. This study provides rational design concepts from catalyst to equipment amelioration by combining promoter regulation and ex situ water removal, efficiently catalyzing CO2 into valuable chemical feedstocks with industrial potential.
中文翻译：
尖晶石结构催化剂以超高产率催化CO2加氢成全谱烯烃。
尖晶石状ZnFe 2 O 4是为催化CO 2加氢而量身定制的合成方法，可在三级反应器系统中实现超光谱全烯烃的高收率（1858.1 g kg cat -1 h -1）。这项研究提供了合理的设计概念，从催化剂到设备改进，方法是将促进剂调节和异位除水相结合，有效地将CO 2催化成具有工业潜力的有价值的化学原料。
更新日期：2020-08-14
中文翻译：
尖晶石结构催化剂以超高产率催化CO2加氢成全谱烯烃。
尖晶石状ZnFe 2 O 4是为催化CO 2加氢而量身定制的合成方法，可在三级反应器系统中实现超光谱全烯烃的高收率（1858.1 g kg cat -1 h -1）。这项研究提供了合理的设计概念，从催化剂到设备改进，方法是将促进剂调节和异位除水相结合，有效地将CO 2催化成具有工业潜力的有价值的化学原料。
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