659
成果及论文
- J.-J. Wang, L. Tang, Y. Xiao, W.-B. Wu, G. Wang,* and J.-J. Feng* "Switching between the [2π+2σ] and Hetero-[4π+2σ] Cycloaddition Reactivity of Bicyclobutanes with Lewis Acid Catalysts Enables the Synthesis of Spirocycles and Bridged Heterocycles" Angew. Chem. Int. Ed., 2024, DOI: 10.1002/anie.202405222.
- J.-L. Zhou, Y. Xiao, L. He, X.-Y Gao, X.-C. Yang, W.-B. Wu, G. Wang, J. Zhang,* and J.-J. Feng* "Palladium-Catalyzed Ligand-Controlled Switchable Hetero-(5 + 3)/Enantioselective [2σ+2σ] Cycloadditions of Bicyclobutanes with Vinyl Oxiranes" J. Am. Chem. Soc. 2024, DOI: 10.1021/jacs.4c01851.
- X. Su, G. Li, L. He, S. Chen, X. Yang, G. Wang,* S. Li* "Nickel-Catalyzed, silyl-directed, ortho-borylation of arenes via an unusual Ni(II)/Ni(IV) catalytic cycle" Submitted.
- L. Dai, Y. Fu, M. Wei, F. Wang, B. Tian, L. Zhang, G. Wang*, S. Li* and M. Ding* "Harnessing Electro-Descriptors for Mechanistic and Predictive Data Analysis of Photocatalytic Organic Reactions" J. Am. Chem. Soc. 2024, DOI: 10.1021/jacs.4c03085.
- Y. Peng, G. Wang,* H. F. T. Klare M. Oestreich* "Ring contraction of saturated cyclic amines and skeletal reorganization of acyclic amines" Angew. Chem. Int. Ed., 2024, DOI: 10.1002/anie.202410483
- Y. Xiao, M. Wei, F. Wu, L. Tang, G. Wang,* and J.-J. Feng* "The Divergent Synthesis of Sulfur-Containing Bridged Cyclobutanes by Lewis Acid Catalyzed Formal Cycloadditions of Pyridinium 1,4-Zwitterionic Thiolates and Bicyclobutanes" Angew. Chem. Int. Ed., 2024, DOI: 10.1002/anie.202408578
- Y. Xiao,‡ J.-L. Zhou,‡ M. Wei,‡ F. Wu, L.Tang, T.-T. Xu, Y. Cai, W.-B. Wu, G. Wang,* J.-J. Feng* "Modular Access to Fused 2-Azabicyclo[2.1.1]hexanes: Lewis Acid Catalyzed Dearomative [3+2] Cycloaddition of Benzazoles with Bicyclobutanes" In revision.
- F. Wu,+ W.-B. Wu,+ Y. Xiao, Z. Li, L. Tang, H.-X. He, X.-C. Yang, J.-J. Wang, Y. Cai, T.-T. Xu, J.-. Tao, G. Wang,* and J.-J. Feng* "Zinc-Catalyzed Enantioselective Formal (3+2) Cycloadditions of Bicyclobutanes with Imines: Catalytic Asymmetric Synthesis of Azabicyclo[2.1.1]hexanes and Beyond" Under review.
- J. Cao, L. Gao, G. Wang*, S. Li* "Visible Light Catalyzed Arylsilylation of Alkenes to Construct Silicon-Containing 1,1-Diaryl Moieties" Green Chem. 2024, 26, 4785-4791.
- L. He,+ Y. Fu,+ S. Hou,+ G. Wang*, J. Zhao, Y. Xing, S. Li and J. Ma* "Reaction Condition- and Functional Group-Specific Knowledge Discovery: Data- and Computation-based Analysis on Transition-Metal-Free Transformation of Organoborons" Artificial Intelligence Chemistry 2024, 2, 100034.
- G. Wang,+ X. Wu,+ B. Xin,+ X. Gu, G. Wang, Y. Zhang, J. Zhao, X. Cheng, C. Chen* and J. Ma* "Machine Learning in Unmanned Systems for Chemical Synthesis" Molecules 2023, 28, 2232.
- L. Gao, X. Liang, L. He, G. Li, S. Chen, J. Cao, J. Ma, G. Wang* and S. Li* "Base-mediated C–B bond activation of benzylic boronate for the rapid construction of b-silyl/boryl functionalized 1,1-diarylalkanes from aromatic alkenes" Chem. Sci. 2023, 14, 11881.
- Y. Xiao, L. Tang, T.-T. Xu, J.-Y.-H. Sheng, Z. Zhou, L. Yue, G. Wang,* M. Oestreich* and J.-J. Feng* "Atom-economic and stereoselective catalytic synthesis of fully substituted enol esters/carbonates of amides in acyclic systems enabled by boron Lewis acid catalysis" Chem. Sci. 2023, 14, 5608.
- G. Li, Z. Li, L. Gao, S. Chen, G. Wang* and S. Li* "Combined molecular dynamics and coordinate driving method for automatically searching complicated reaction pathways" Phys. Chem. Chem. Phys. 2023, 25, 23696.
- X. Liu, Y. Wang, S. Chen, Q. Jia, G. Wang* and S. Li,* "Direct benzylic polychlorination of (poly)azines with N-chlorosuccinimide" Org. Chem. Front. 2023, 10, 3336.
- S. Jin, Y. Wang, Y. Tang, J.-Y. Wang, T. Xu, J. Pan, S. Zhang, Q. Yuan, A. U. Rahman, J. D. McDonald, G. Wang*, S. Li and G. Li*, "Orientational Chirality, its Asymmetric Control and Computational Study" Research 2022, 2022, 0012.
- W. Zou, M. Yang, L. He, G. Wang* and S. Li* "Mechanistic insights into the metal-free deoxygenative borylation of ketones and aldehydes with bis(catecholato)diborane" Chem. Eur. J., 2022, e202203526.
- J. Cao, L. Gao, G. Wang* and S. Li* "Pyridine-Catalyzed Decarboxylative Homolytic Substitution of N-hydroxyphthalimide Ester with Ph2X2(X=S, Se)" Eur. J.Org. Chem. 2022, e202201290.
- P.-W. Long, G. Wang*, H. F. T. Klare, and M. Oestreich* "Silylium-Ion-Promoted Skeletal Reorganization of β-Silylated Cyclopropanes Bearing an Allyl Group at the Silicon Atom Coupled with Intermolecular Formation of a Quaternary Carbon Atom" ACS Catal. 2022, 12, 12310.
- L. Gao, X. Liu, G. Li, S. Chen, J. Cao, G. Wang* and S. Li* "1,2-Silylpyridylation Reaction of Aryl Alkenes with Silylboronate" Org. Lett. 2022, 24, 5698.
- W. Zou, L. Gao, J. Cao, Z. Li, G. Li, G. Wang* and S. Li* "Mechanistic Insight into Hydroboration of Imines from Combined Computational and Experimental Studies" Chem. Eur. J. 2022, 28, e202104004.
- J. Cao, G. Li, G. Wang*, L. Gao and S. Li* "Iodoperfluoroalkylation of unactivated alkenes via pyridine-boryl radical initiated atom-transfer radical addition" Org. Biomol. Chem. 2022, 20, 2857.
- G. Wang+, X. Su+, L. Gao+, X. Liu, G. Li and S. Li* "Borane-Catalyzed Selective Dihydrosilylation of Terminal Alkynes: Reaction Development and Mechanistic Insight" Chem. Sci. 2021, 12, 10883.
- H. Chen, L. Gao, X. Liu, G. Wang* and S. Li* "B(C6F5)3-Catalyzed Hydroarylation of Aryl Alkynes for the Synthesis of 1,1-Diaryl and Triaryl Substituted Alkenes" Eur. J. Org. Chem. 2021, 5238.
- H. Chen, M. Yang, G. Wang*, L. Gao, Z. Ni, J. Zou, and S. Li* "B(C6F5)3‑Catalyzed Sequential Additions of Terminal Alkynes to para-Substituted Phenols: Selective Construction of Congested Phenol-Substituted Quaternary Carbons" Org. Lett. 2021, 23, 5533.
- L. Gao+, H. Zhang+, X. Liu, G. Wang,* and S. Li* "Mechanistic insights into the dearomative diborylation of pyrazines: a radical or non-radical process?" Dalton Trans., 2021, 50, 6982.
- H. Fang+, G. Wang,+ and M. Oestreich* "Mild reductive rearrangement of oximes and oxime ethers to secondary amines with hydrosilanes catalyzed by B(C6F5)3" Org. Chem. Front., 2021, 8, 3280.
- L. Gao,+ G. Wang+, H. Chen, J. Cao, X. Su, X. Liu, M. Yang, X. Cheng S. Li* "Metal-free reductive coupling of aliphatic aldehydes/ketones with 4-cyanopyridines: expanded scope and mechanistic studies" Org. Chem. Front., 2020, 7, 2744.
- T. Xie+, G. Wang+, Y. Wang, W. Rao, H. Xu, S. Li*, Z. Shen* and X. Chu* "Selective Quadruple C(sp3)-F Functionalization of Polyfluoroalkyl Ketones" iScience 2020, 23, 101259.
- L. Gao+, G. Wang+, J. Cao, H. Chen, Y. Gu, X. Liu, X. Cheng, J. Ma, and S. Li* "Lewis Acid-Catalyzed Selective Reductive Decarboxylative Pyridylation of N-Hydroxyphthalimide Esters: Synthesis of Congested Pyridine-Substituted Quaternary Carbons" ACS Catal., 2019, 9, 10142.
- P. Gao+, G. Wang+, L. Xi, M. Wang, S. Li,* and Z. Shi* "Transition-Metal-Free Defluorosilylation of Fluoroalkenes with Silylboronates" Chin. J. Chem., 2019, 37, 1009.
- G. Wang+, L. Gao+, H. Chen, X. Liu, J. Cao, S. Chen, X. Cheng and S. Li* "Borane-Catalyzed Chemoselective Hydroarylation of 1,3-Dienes with Phenols" Angew. Chem. Int. Ed. 2019, 58, 1694.
- M. Yang+, G. Wang+, J. Zou and S. Li*, "Mechanistic Insight Into the AuCN Catalyzed Annulation Reaction of Salicylaldehyde and Aryl Acetylene: Cyanide Ion Promoted Umpolung Hydroacylation/Intramolecular Oxa-Michael Addition Mechanism" Front. Chem. 2019, 7, 557.
- L. Gao+, G. Wang+, J. Cao, D. Yuan, X. Cheng, X. Guo, S. Li* "Organocatalytic decarboxylative alkylation of N-hydroxy-phthalimide esters enabled by pyridine-boryl radicals" Chem. Commun., 2018, 54, 11534.
- J. Cao+, G. Wang+, L. Gao, X. Cheng and S. Li* "Organocatalytic reductive coupling of aldehydes with 1,1-diarylethylenes using an in situ generated pyridine-boryl radical" Chem. Sci., 2018, 9, 3664.
- J. Hu+, G. Wang+, S. Li* and Z. Shi* "Selective C-N Borylation of Alkyl Amines Promoted by Lewis Base" Angew. Chem. Int. Ed. 2018, 57, 15227.
- D. Yan+, G. Wang+, F. Xiong+, W. Sun, Z. Shi, Y. Lu,* S. Li* and J. Zhao,* "A selenium-catalysed para-amination of phenols" Nat. Comm. 2018, 9, 4293.
- M. Yang, L. Yang, G. Wang, Y. Zhou*, D. Xie and S. Li*, "Combined Molecular Dynamics and Coordinate Driving Method for Automatic Reaction Pathway Search of Reactions in Solution" J. Chem. Theory Comput. 2018, 14, 5787.
- G. Wang, J. Cao, L. Gao, W. Chen, W. Huang, X. Cheng* and S. Li* "Metal-Free Synthesis of C-4 Substituted Pyridine Derivatives Using Pyridine-boryl Radicals via a Radical Addition/Coupling Mechanism: A Combined Computational and Experimental Study" J. Am. Chem. Soc. 2017, 139, 3904.
- M. Yang, J. Zou, G. Wang and S. Li*, "Automatic Reaction Pathway Search via Combined Molecular Dynamics and Coordinate Driving Method" J. Phys. Chem. A, 2017, 121, 1351.
- P. Xu, G. Wang, Z. Wu, S. Li* and C. Zhu* "Rh(III)-catalyzed double C–H activation of aldehyde hydrazones: a route for functionalized 1H-indazole synthesis" Chem. Sci., 2017, 8, 1303.
- W. Chen, H. Tao, W. Huang, G. Wang, S. Li,* X. Cheng,* and G. Li, "Hantzsch Esterasa Photosensitizer for the Visible-Light-Induced Debromination of Vicinal Dibromo Compounds" Chem. Eur. J., 2016, 22, 9546.
- G. Wang, H. Zhang, J. Zhao, W. Li, J. Cao, C. Zhu* and S. Li* "Homolytic Cleavage of a B−B Bond by the Cooperative Catalysis of Two Lewis Bases: Computational Design and Experimental Verification" Angew. Chem. Int. Ed. 2016, 55, 5985.