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成果及论文

在Nature Mater., Phys. Rev. Lett., Angew. Chem. Int. Ed., ACS Nano, Nano Lett., Adv. Funct. Mater., Carbon, Nano Res.等期刊发表论文50余篇;其中第一作者发表在Nature Materials上的论文报道了世界上最长碳链的成功制备和性能研究,受到了审稿人的极高评价和科学界极大的关注(上百家国内外媒体报道,如Sciencedaily, C&EN, MRS, MailDaily,科技日报的头版头条和主编点评,等等),被ACS Central Sciences评为2016年度化学界的五大世界纪录之一,目前是所在碳链领域被引用最快的论文之一。

Research ID:http://www.researcherid.com/rid/D-5367-2012

Publons: https://publons.com/researcher/1357199/lei-shi/

Google Scholar: https://scholar.google.com/citations?hl=zh-CN&user=kX4FyXAAAAAJ

 

*通讯作者        #共同一作

2024:

62.  The resonant Raman response of confined carbyne is solely driven by anharmonic interactions. Submitted (2024). Emil Parth*, Andrea Corradini, Weili Cui, Davide Romanin, Christin Schuster, Clara Freytag, Lei Shi, Kazuhiro Yanagi, Matteo Calandra, Thomas Pichler. DOI: 10.21203/rs.3.rs-5247129/v1

61. Universal Vibrational Anharmonicity in Carbyne-like Materials. Submitted (2024). Johannes M. A. Lechner, Pietro Marabotti, Lei Shi, Thomas Pichler, Carlo Spartaco Casari, Sebastian Heeg*.

60. Confined synthesis and thermal conductivity of deuterated graphene nanoribbons. Accepted, Carbon119841 (2024)  https://doi.org/10.1016/j.carbon.2024.119841Yingzhi Chen, Wendi Zhang, Kunpeng Tang, Kecheng CaoLei Shi*, Guowei Yang.

59. Precursor-driven confined synthesis of highly pure 5-armchair graphene nanoribbons. Small MethodsDOI: 10.1002/smtd.202401168 (2024). Weili Cui, Wendi Zhang, Kunpeng Tang, Yingzhi Chen, Kecheng Cao*, Lei Shi*, Guowei Yang.

58. Sp1-hybridized linear and cyclic carbon chainChinese Chemical Letters, DOI: https://doi.org/10.1016/j.cclet.2024.110466 (2024). Huiju Cao, Lei Shi*.

57. Advanced 1D heterostructures based on nanotubes templates and moleculesChemical Society Reviews, 53, 8457-8512 (2024) Charlotte Allard, Laurent Alvarez, Jean-Louis Bantignies, Nedjma Bendiab, Sofie Cambré, Stephane Campidelli, Jeffrey A. Fagan, Emmanuel Flahaut, Benjamin Flavel, Frederic Fossard, Etienne Gaufrès*, Sebastian Heeg, Jean-Sebastien Lauret, Annick Loiseau, Jean-Baptiste Marceau, Richard Martel, Laetitia Marty, Thomas Pichler, Christophe Voisin, Stephanie Reich, Antonio Setaro, Lei Shi, Wim Wenseleers. (The authors are listed in alphabetical order)


56. 2D Growth of BiSCl as Anisotropic Photodetector with Ultrahigh Responsivity and DetectivityAdvanced Optical Materials, 12, 2400664 (2024). Ziheng Lin, Xuanhao Yuan, Ruize Wang, Yan Li, Lei Shi, Weili Cui, Lishan Liang, Zihao Huang, Fei Tian, Yong Sun*, Chengxin Wang*.

55. Encapsulation and Evolution of Polyynes Inside Single-Walled Carbon Nanotubes. Nanomaterials, 14, 966 (2024). Kunpeng Tang, Yinong Li, Yingzhi Chen, Weili Cui, Zhiwei Lin, Yifan Zhang*, Lei Shi*.

54. Significant electron-phonon coupling in nanographene confined in single-walled carbon nanotubes due to the large amplitude of radial breathinglike vibrationsPhysical Review B, 109, 195413 (2024) Bingze Wu, Mingfeng Zhu, Chunguang Zhai, Yaping Zhao, Yexuan Meng, Jiajun Dong, Xuan Li, Ran Liu, Kunpeng Tang, Lei Shi*, Bertil Sundqvist, Mingguang Yao*.

53. Mixed-ligand-functionalized silicon-germanium alloy nanocrystals with improved carrier mobilitiesNanoscale, 16, 6516-6521 (2024) Linfeng Wei, Haoyuan Zhang, Lei ShiZhenyu Yang*.

52. A robust synthesis route of confined carbyne. Nano Research, 17, 62746280 (2024) Yanghao Feng#Wendi Zhang#, Kunpeng Tang, Yingzhi Chen, Jiou Zhang, Kecheng Cao*, Weili Cui*, Lei Shi*.

51. Unraveling the governing properties of confined carbyne through the interaction with its carbon nanotube host. Carbon, 219,118784 (2024) Weili Cui, Paola Ayala, Thomas Pichler*, Lei Shi*.


2023:

50. A Simulation of the Effect of External and Internal Parameters on the Synthesis of a Carbyne with More than 6000 Atoms for Emerging Continuously Tunable Energy Barriers in CNT-Based Transistors. Nanomaterials 13, 1048 (2023)  Chi Ho Wong*, Yan Ming Yeung, Xin Zhao, Wing Cheung Law, Chak-yin Tang, Chee Leung Mak, Chi Wah Leung, Lei Shi, Rolf Lortz.

49. Microwave heating as a universal method to transform confined molecules into armchair graphene nanoribbonsNano Research16(7), 1064410651 (2023) Haoyuan Zhang#, Yingzhi Chen#, Kunpeng Tang#, Ziheng Lin, Xuan Li, Hongwei Zhang, Yifan Zhang, Chi Ho Wong, Chi Wah Leung, Chee Leung Mak, Yuan Hu, Weili Cui*, Kecheng Cao*, Lei Shi*.



48. 1D nanoribbons of 2D materialsProgress in Chemistry, 35, 88104 (2023) Xuan Li#, Jiongpeng Huang#, Yifan Zhang, Lei Shi*. 


2022:

47. Highly sensitive and selective formaldehyde gas sensors based on polyvinylpyrrolidone/nitrogen-doped double-walled carbon nanotubesSensors22, 9329 (2022) Thanattha Chobsilp, Thotsaphon Trirujirapapong, Visittapong Yordsri, Alongkot Treetong, Saowaluk Inpaeng, Karaked Tedsree, Paola Ayala, Thomas Pichler, Lei Shi, Worawut Muangrat*. 

46. Nitrogen-tailored quasiparticle energy gaps of polyynes. Chinese Physics B, 31, 123102 (2022) Kan Zhang, Jiling Li, Peitao Liu, Guowei Yang, Lei Shi*. 

45. Ultra-clean isotope engineered double-walled carbon nanotubes as tailored hosts to trace the growth of carbyne. Advanced Functional Materials, 32, 2206491 (2022) Weili Cui*, Ferenc Simon, Yifan Zhang, Lei Shi*, Paola Ayala, Thomas Pichler*. 

44. Unravelling the Complete Raman Response of Graphene Nanoribbons Discerning the Signature of Edge Passivation. Small Methods, 6, 2200110 (2022) Valeria Milotti, Claudia Berkmann, Jorge Laranjeira, Weili Cui, Kecheng Cao, Yifan Zhang, Ute Kaiser, Kazuhiro Yanagi, Manuel Melle-Franco, Lei Shi*, Thomas Pichler*, Paola Ayala*.

43. Comment on “Anharmonicity and Universal Response of Linear Carbon Chain Mechanical Properties under Hydrostatic Pressure”Physical Review Letters, 128, 219601 (2022) Enlai Gao, Ke Zhou, Lei Shi*, Zhiping Xu*. 

42. Tip-enhanced Stokes–anti-Stokes scattering from carbyneNano Letters, 22 (8), 3260–3265 (2022) Cla Duri Tschannen*, Martin Frimmer, Thiago L. Vasconcelos, Lei Shi, Thomas Pichler, Lukas Novotny. 

41. Magnetic nanoribbons with embedded cobalt grown inside single-walled carbon nanotubesNanoscale, 14, 1978–1989 (2022) Denis M. Krichevsky, Lei Shi, Vladimir S. Baturin, Dmitry V. Rybkovsky, Yangliu Wu, Pavel V. Fedotov, Elena D. Obraztsova, Pavel O. Kapralov, Polina V. Shilina, Kayleigh Fung, Craig T. Stoppiello, Vladimir I. Belotelov, Andrei Khlobystov, Alexander I. Chernov*. 

40. Electronic structure of confined carbyne from joint wavelength-dependent resonant Raman spectroscopy and density functional theory investigations. Carbon, 189, 276283 (2022) Miles Martinati, Wim Wenseleers*, Lei Shi, Saied Md Pratik, Philip Rohringer, Weili Cui, Thomas Pichler, Veaceslav Coropceanu, Jean-Luc Brédas, Sofie Cambré*. 



39. Carbon nanotube-dependent synthesis of armchair graphene nanoribbonsNano Research,  15(3), 1709−1714 (2022) Yifan Zhang, Kecheng Cao, Takeshi Saito, Hiromichi Kataura, Hans Kuzmany, Thomas Pichler, Ute Kaiser, Guowei Yang*,  Lei Shi*.


2021:

38. Unraveling the excitonic transition and associated dynamics in confined long linear carbon-chains with time-resolved resonance Raman scatteringLaser & Photonics Reviews, 15, 2100259 (2021) Jingyi Zhu*, Robin Bernhardt, Weili Cui, Raphael German, Julian Wagner, Boris V. Senkovskiy, Alexander Grüneis, Thomas Pichler, Yuxuan Li, Xueyang Li, Kaifeng Wu*, Rulin Liu, Xi Zhu, Paul H. M. Van Loosdrecht*, Lei Shi*.


37. Anti-Stokes Raman scattering of single carbyne chains. ACS Nano15(7), 12249–12255 (2021) Cla Duri Tschannen*, Martin Frimmer, Georgy Gordeev, Thiago L. Vasconcelos, Lei Shi, Thomas Pichler, Stephanie Reich, Sebastian Heeg, Lukas Novotny. 

36. Photothermal synthesis of confined carbyneCarbon182, 348–353 (2021) Lei Shi*, Ryosuke Senga, Kazu Suenaga, Johnny Chimborazo, Paola Ayala, Thomas Pichler*. 封面文章 Front cover

35. Isotopic labeling of confined carbyneAngewandte Chemie-International Edition, 60, 9897–9901 (2021) Weili Cui, Lei Shi*, Kecheng Cao, Ute Kaiser, Takeshi Saito, Paola Ayala, Thomas Pichler*.

34. Pressure-tailored synthesis of confined linear carbon chainsJournal of Applied Physics, 129, 064302 (2021) Xuan Li, Yifan Zhang, Yangliu Wu, Lei Shi*. 

33. Toward Confined Carbyne with Tailored Properties. Nano Letters, 21, 1096–1101 (2021).  Lei Shi*, Ryosuke Senga, Kazu Suenaga, Hiromichi Kataura, Takeshi Saito, Alejandro Perez Paz*, Angel Rubio*, Paola Ayala, Thomas Pichler*.

32. One-Dimensional New Carbon allotrope: Carbon Chain. Progress in Chemistry3(2), 187-198 (2021). Jun Jin, Ziheng Lin, Lei Shi*.

31. Well-defined sub-nanometer graphene ribbons synthesized inside carbon nanotubes. Carbon, 171, 221-229, (2021). Hans Kuzmany#*, Lei Shi#*, Miles Martinati, Sofie Cambré, Wim Wenseleers, Jeno Kürti, János Koltai, Gergo Kukucska, Kecheng Cao, Ute Kaiser, Takeshi Saito, Thomas Pichler. 


2020:

30. Raman scattering cross section of confined carbyne. Nano Letters, 20, 6750−6755 (2020). Cla Duri Tschannen, Georgy Gordeev, Stephanie Reich, Lei Shi, Thomas Pichler, Martin Frimmer, Lukas Novotny, Sebastian Heeg*. 

29. A review of linear carbon chainsChinese Chemical Letters31, 1746−1756 (2020) Kan Zhang#, Yifan Zhang#Lei Shi*.

28. Band-gap engineering and structure evolution of confined linear carbon chains@double-walled carbon nanotubes under pressureCarbon, 159, 266−272 (2020)  Xigui Yang#, Chaofan Lv#, Zhen Yao, Mingguang Yao*, Jinxu Qin, Xing Li, Lei Shi*, Mingrun Du, Bingbing Liu, Chong-Xin Shan*.


2019:

27. Oxidation stability of confined linear carbon chains, carbon nanotubes, and graphene nanoribbons as 1D nanocarbons Nanoscale, 11, 1525315258 (2019) Weili Cui, Takeshi Saito, Paola Ayala, Thomas Pichler, Lei Shi*

26.Towards controllable inner chirality in double-walled carbon nanotubes. Applied Physics Letters115, 103102 (2019)  Johnny Chimborazo, Takeshi Saito, Thomas Pichler, Lei Shi*, Paola Ayala*.

25. Wall- and hybridisation- selective synthesis of nitrogen-doped double-walled carbon nanotubes. Angewandte Chemie International Edition, 30, 1027610280 (2019) Marco Carini, Lei Shi, Thomas W. Chamberlain, Meng Liu, Giovanni Valenti, Manuel Melle-Franco, Francesco Paolucci, Andrei N. Khlobystov*, Thomas Pichler*, Aurelio Mateo-Alonso*. 

24. Towards a predominant substitutional bonding environment in B-doped single-walled carbon nanotubes. ACS Omega, 4, 1941–1946 (2019) Carlos Reinoso, Claudia Berkmann, Lei Shi, Alexis Debut, Kazuhiro Yanagi, Thomas Pichler, Paola Ayala*

-----------------------------------分界线:以上为中山大学为作者单位(之一)的论文

 

2018:

23. Templated Direct growth of ultra-thin double-walled carbon nanotubes. Nanoscale, 10, 21254−21261(2018) Lei Shi*, Jinquan Wei, Takeshi Saito, Kecheng Cao, Ute Kaiser, Paola Ayala, Thomas Pichler. 

22. Very-high boron-doping on single-walled carbon nanotubes from a solid precursorCarbon, 140, 259−264 (2018) C. Reinoso, Lei Shi, Oleg Domanov, Philip Rohringer, Thomas Pichler, Paola Ayala*.

21. Carbon nanotube chirality determines properties of encapsulated linear carbon chainsNano Letters, 18 (9), 5426−5431 (2018) Sebastian Heeg, Lei Shi, L. V. Poulikakos, Thomas Pichler, Lukas Novotny*.  

20. Extracting linear carbon chains to unravel the role of host carbon nanotubesACS Nano, 12 (8), 8477–8484 (2018) Lei Shi, Kazuhiro Yanagi, Kecheng Cao, Ute Kaiser, Paola Ayala, Thomas Pichler*. 

19. Raman resonance profile of an individual confined linear carbon chainCarbon, 139, 581−585 (2018) Sebastian Heeg, Lei Shi, Lisa V. Poulikakos, Thomas Pichler, Lukas Novotny*. 

18. Unravel the active site in nitrogen-doped double-walled carbon nanotubes for nitrogen dioxide gas sensor. Physica Status Solidi (a), 1800004 (2018) Worawut Muangrat, Winadda Wongwiriyapan, Visittapong Yordsri, Thanattha Chobsilp, Saowaluk Inpaeng, Chaisak Issro, Oleg Domanov, Paola Ayala, Thomas Pichler, Lei Shi*.  

17. Isotope effect on the quantum thermal transport of carbyneApplied Physics Letters, 112 (9), 091906 (2018) Yu Wu, Jing Zhao, Guangyu Sun, Lei Shi*.

 

2017:

16. Electronic band gaps of confined linear carbon chains ranging from polyyne to carbyne. Physical Review Materials 1, 075601 (2017) Lei ShiPhilip Rohringer, Marius Wanko, Angel Rubio, Sören Waßerroth, Stephanie Reich, Sofie Cambré, Wim Wenseleers, Paola Ayala, Thomas Pichler*.

15. The growth of new extended carbon nanophases from ferrocene inside single-walled carbon nanotubesphysica status solidi (RRL) - Rapid Research Letters, 8, 1700158 (2017) Hans Kuzmany*, Lei Shi*, Jeno Kürti, Janos Koltai, Andrey Chuvilin, Takeshi Saito, Thomas Pichler.

14. 2D-heterostructures derived from MoS2-templated, cobalt-containing conjugated microporous polymer sandwiches for oxygen reduction reaction and electrochemical energy storageChemElectroChem, 4, 709−715 (2017) Kai Yuan, Xiaodong Zhuang*, Ting Hu, Lei Shi, Stavroula Sfaelou, Ulrike Polnick, Michael Forster, Thomas Pichler, Thomas Riedl, Xinliang Feng, Yiwang Chen*, Ullrich Scherf*.

13.Nitrogen-doped porous carbon/graphene nanosheets derived from two-dimensional conjugated microporous polymer sandwiches with promising capacitive performanceMaterials Chemistry Frontiers, 1, 278−285 (2017)  Kai Yuan, Ting Hu, Yazhou Xu, Robert Graf, Lei Shi, Michael Forster, Thomas Pichler, Thomas Riedl, Yiwang Chen*, Ullrich Scherf*. 

 

2016:

12.Polyyne electronic and vibrational properties under environmental interactionsPhysical Review B, 94, 195422 (2016)  Marius Wanko, Seymur Cahangirov, Lei Shi, Philip Rohringer, Zachary J. Lapin, Lukas Novotny, Paola Ayala, Thomas Pichler,  Angel Rubio.

11. Confined linear carbon chains as a route to bulk carbyneNature Materials, 15, 634−639; (2016) Lei ShiPhilip Rohringer, Kazu Suenaga, Yoshiko Niimi, Jani Kotakoski, Jannik C. Meyer, Herwig Peterlik, Marius Wanko, Seymur Cahangirov, Angel Rubio, Zachary J. Lapin, Lukas Novotny, Paola Ayala, Thomas Pichler*. (ESI: Highly cited paper)

This paper has been recognized as record breaking result in chemistry (ACS Central Sciences2, 489(2016); DOI: 10.1021/acscentsci.6b00211). Awards to two compositions (UK and AT) based on the story of “Chain Growth” in the international composer competition “Sounds of Matter”.

10.Selective enhancement of inner tube photoluminescence in filled double-walled carbon nanotubesAdvanced Functional Materials, 26, 4874–4881 (2016) Philip Rohringer, Lei Shi, Paola Ayala, Thomas Pichler*.

 

2015:

9. Straightforward generation of pillared, microporous graphene frameworks for use in supercapacitorsAdvanced Materials, 27, 6714–6721 (2015) Kai Yuan, Yazhou Xu, Johannes Uihlein, Gunther Brunklaus, Lei Shi, Ralf Heiderhoff, Mingming Que, Michael Forster, Thomas Chassé, Thomas Pichler, Thomas Riedl, Yiwang Chen*, Ullrich Scherf*.

8. Nanofibrous and graphene-templated conjugated microporous polymer materials for flexible chemosensors and supercapacitorsChemistry of Materials, 27, 7403–7411 (2015) Kai Yuan, Peiyao Guo-Wang, Ting Hu, Lei Shi, Rong Zeng, Michael Forster, Thomas Pichler, Yiwang Chen*, Ullrich Scherf*.

7.Raman and XPS analyses of pristine and annealed N-doped double-walled carbon nanotubesPhysica Status Solidi (b), 2522558–2563 (2015) Lei Shi*, Markus Sauer, Oleg Domanov, Philip Rohringer, Paola Ayala, Thomas Pichler.

6. The origin of nondispersive Raman lines in the Dband region for ferrocene@ HiPco SWCNTs transformed at high temperaturesPhysica Status Solidi (b), 252, 2530–2535 (2015) Hans Kuzmany*, Lei Shi, Thomas Pichler, Jeno Kürti, Janos Koltai, Ferdinand Hof, Takeshi Saito.

 

Before 2015:

5. Purification, separation and extraction of inner tubes from double-walled carbon nanotubes by tailoring density gradient ultracentrifugation using optical probesCarbon, 74, 282–290 (2014) Philip Rohringer, Lei Shi, Xianjie Liu, Kazuhiro Yanagi, Thomas Pichler*.

4. Nondispersive Raman lines in the D-band region for ferrocene functionalized carbon nanotubes. Physica Status Solidi (b), 251, 2457–2460 (2014) Hans Kuzmany*, Lei Shi, Thomas Pichler, C. Kramberger, Alexander Chernov, Xianjie Liu. 

3.Carbon nanotubes from enhanced direct injection pyrolytic synthesis as templates for long linear carbon chain formation. Physica Status Solidi (b), 250, 2611–2615 (2013) Lei Shi*, Philip Rohringer, Paola Ayala, Takeshi Saito, Thomas Pichler. 

2. Ultra-thin double-walled carbon nanotubes: A novel nanocontainer for preparing atomic wiresNano Research, 4, 759–766 (2011) Lei Shi, Leimei Sheng*, Liming Yu, Kang An, Yoshinori Ando, Xinluo Zhao*.

1. Effective and efficient purification of single-wall carbon nanotubes based on hydrogen treatment.  Chemical Physics Letters, 502, 101–106 (2011) Leimei Sheng, Lei Shi, Kang An, Liming Yu, Yoshinori Ando, Xinluo Zhao*. 


书籍(章节):

1. Synthesis of Confined Carbyne inside Carbon Nanotubes by Thermal Annealing. Weili Cui, Lei Shi*. Page 247-266, Emerging Carbyne——Truly One-Dimensional Form of Carbon. Edited By Yahachi Saito, New York, Jenny Stanford Publishing, 11 October 2024, eBook ISBN 9781003510369. DOI: https://doi.org/10.1201/9781003510369


授权发明专利(近五年):

1. 一种合成碳链的方法;申请日:2022.08.11,专利号ZL202210964082.6申请人:中山大学,发明人:石磊;陈颖芝;张宏伟;唐鲲鹏

2. 一种提高碳链产率的方法;申请日:2022.08.01,专利号:ZL202210917268.6,申请人:中山大学,发明人:石磊;张纪瓯;李璇

3. 一种一维碳链的制备方法;申请日:2019.11.21,专利号:ZL201911151182.1,申请人:中山大学,发明人:石磊;张一帆;杨国伟;刘璞;王建兴

4.一种石墨烯-钨酸铋的制备方法及其应用申请日:2019.10.15,专利号:ZL201910979575.5申请人:中山大学,发明人:刘璞;魏子晔;李振邦;王建兴;刘才超;石磊;杨国伟

5.一种钨酸铋- 石墨烯- 导电水凝胶的制备方法及其应用申请日:2019.10.15,专利号:ZL201910980260.2申请人:中山大学,发明人:刘璞;魏子晔;李振邦;王建兴;刘才超;杨国伟;石磊

6.钯磷硫微纳颗粒的制备及其在光热领域中的应用申请日:2022.08.24,专利号:ZL202211021236.4申请人:中山大学,发明人:刘璞;李一凡;付国帅;杨国伟;于鹏;石磊