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成果及论文

主要学术论文                                                      

近五年来,本课题组的相关研究成果《Applied Catalysis B: Environmental》《Water Research》等知名刊物上发表论文56篇。如下:

1.       Dongya Li, Shiyu Zuo, Jinquan Wan, Yan Wang*, Zeyu Guan, Zhicheng Yan, Fan Yang, Revealing the synergistic mechanism of generation, release, migration and utilization of reactive oxygen species through tailoring the d-band in metal organic frameworks for water purification [J]. Applied Catalysis B: Environmental, 2023, 328, 122507. IF=24.319,中科院1 TOP

2.       Shiyu Zuo, Yichen Ding, Li Wu, Fan Yang, Zeyu Guan, Su Ding, Dongsheng Xia, Xiaohu Li, Dongya Li*, Revealing the synergistic mechanism of the generation, migration and nearby utilization of reactive oxygen species in FeOCl-MOF yolk-shell reactors [J]. Water Research, 2023, 231,119631. IF=13.400,中科院1 TOP,自然指数期刊)

3.       Meng Li, Dongya Li*, Shasha Li, Jianyun Liu, Huiyuan Deng, Dongsheng Xia*, Novel sludge-sugarcane bagasse mixed biochar as an efficient activator for peroxymonosulfate to degrade bisphenol AF [J]. Chemical Engineering Journal, 2023,462,142114. IF=16.744,中科院1 TOP

4.       Zeyu Guan, Yiming Zhang, Shiyu Zuo, Shibo Zhu, Weishan Wang, Dongya Li*, The synergistic catalytic mechanism between different functional sites of boron/iron on iron oxides in Fenton-like reactions [J]. Separation and Purification Technology, 2023, 312, 123391. IF=9.136,中科院1 TOP

5.       Qihui Wang, Zeyu Guan, Yi Xiong, Dongya Li*, Nanoconfinement-enhanced Fenton-like polymerization via hollow hetero-shell carbon for reducing carbon emissions in organic wastewater purification [J]. Journal of Colloid and Interface Science, 2023, 634: 231-242. IF=9.965,中科院1 TOP

6.       Shiyu Zuo, Yichen Ding, Zeyu Guan, Yiming Zhang, Dongya Li*, Carbon-coated MIL-101(Fe) core–shell tandem mediates the directional conversion of SO4·- to 1O2 to realize efficient removal of bisphenol A [J]. Separation and Purification Technology, 2023, 308, 122871. IF=9.136,中科院1 TOP

7.       Yichen Ding, Shiyu Zuo, Zeyu Guan, Su Ding, Dongya Li*, Surface hydroxyl-riched calcium carbonate and copper oxide composites for Fenton-like removal of bisphenol A [J]. Separation and Purification Technology, 2023, 308, 122912. IF=9.136,中科院1 TOP

8.       Li Wu, Shiyu Zuo, Yi Zhu, Qihui Wang, Dongya Li*, Coordination-driven boron and copper on carbon nitride for peroxymonosulfate activation to efficiently degrade organic contaminants [J]. Separation and Purification Technology, 2023, 312, 123349. IF=9.136,中科院1 TOP

9.       Yi Zhu, Zeyu Guan, Xiaohu Li, Dongsheng Xia, Dongya Li*, Ultrafast short-range catalytic pathway modified peroxymonosulfate activation over CuO with surface oxygen defects for tetracycline hydrochloride degradation [J]. Environmental Research, 2023, 222, 115322. IF=8.431,中科院2区)

10.     Yichen Ding, Shiyu Zuo, Dongya Li*, Zeyu Guan, Fan Yang, Regulating Interlayer Confinement FeOCl for Accelerating Polymerization of Pollutants to Reduce Carbon Emission in Water Purification [J]. ACS Applied Materials & Interfaces, 2023, 5058-5070. IF=10.383,中科院2 TOP

11.     Shiyu Zuo, Zeyu Guan, Yiming Zhang, Fan Yang, Xiaohu Li, Dongya Li*, Bidentate binuclear coordination configuration for peroxymonosulfate catalytic regulation through incorporation of CuFeOx to iron-based metal organic frameworks [J]. Chemical Engineering Journal, 2022, 450 (4), 138461. IF=16.744,中科院1 TOP

12.     Meng Li, Dongya Li*, Zeyu Guan, Qianqian Xu, Yintao Shi, Dongsheng Xia*, Carboxy-functionalized sludge-derived biochar for efficiently activating peroxymonosulfate to degrade bisphenol A [J]. Separation and Purification Technology, 2022, 297, 121525. IF=9.136,中科院1 TOP

13.     Zeyu Guan, Shibo Zhu, Su Ding, Dongsheng Xia, Dongya Li*, Fe–O–Zr in MOF for effective photo-Fenton Bisphenol A degradation: Boosting mechanism of electronic transmission [J]. Chemosphere, 2022, 299:134481.IF=8.943,中科院2 TOP

14.     Shiyu Zuo, Dongya Li*, Zeyu Guan, Fan Yang, Dongsheng Xia. Reactive Oxygen Species Regulation and Synergistic for Effective Water Purification through Fenton-like Catalysis on Single-Atom Cu-N Sites [J]. Journal of Materials Chemistry A, 2022, 10(19),10503-10513. IF=14.511,中科院1 TOP

15.     Shiyu Zuo, Dongya Li*, Zeyu Guan, Fan Yang, Junqi Song, Haiming Xu, Dongsheng Xia, Huanxuan Li, Xiaohu Li. A Directional Built-in Electric Field Mediates the Electron Transfer Synergy Mechanism of Radicals/Nonradicals Pathway in FeOCl-CuO [J]. Chemical Engineering Journal, 2022, 430: 133004. IF=16.744,中科院1 TOP

16.     Shiyu Zuo, Dongya Li*, Zeyu Guan, Fan Yang, Dongsheng Xia, Mingzhi Huang. Utilization of sewage resources through efficient solar-water evaporation by single-atom Cu sites [J]. Carbon, 2022, 187: 207-215. IF=11.307,中科院1TOP

17.     Qihui Wang, Zeyu Guan, Su Ding, Dongsheng Xia, Dongya Li*. Tuning the Surface Electronic State by the introduction of Mn on Fe2O3 to boost the Activity of Peroxymonosulfate[J]. Separation and Purification Technology, 2022: 120625. IF=9.136,中科院1 TOP

18.     Shiyu Zuo, Dongya Li*, Zeyu Guan, Yi Zhu, Mengjie Pu, Dongsheng Xia. Rapid electron transfer boosts CuO-Mediated nonradical oxidation pathways for efficient removal of Bisphenol A[J]. Journal of Cleaner Production, 2022: 130480. IF=11.072,中科院1 TOP

19.     Weishan Wang, Dongya Li*, Shiyu Zuo, Zeyu Guan, Haiming Xu, Su Ding, Dongsheng Xia. Discarded-leaves derived biochar for highly efficient solar water evaporation and clean water production: The crucial roles of graphitized carbon[J]. Colloids and Surfaces A: Physicochemical and Engineering Aspects, 2022: 128337. IF=5.518,中科院2区)

20.     Yichen Ding, Dongya Li*, Shiyu Zuo, Zeyu Guan, Su Ding. Boron-doping accelerated Cu (II)/Cu (I) cycle for enhancing peroxymonosulfate activation [J]. Separation and Purification Technology, 2022, 282: 120086. IF=9.136,中科院1 TOP

21.     Shiyu Zuo, Dongya Li*, Zeyu Guan, Fan Yang, Haiming Xu, Dongsheng Xia, Jinquan Wan. Tailored dBand Facilitating in Fe Gradient Doping CuO Boosts Peroxymonosulfate Activation for High Efficiency Generation and Release of Singlet Oxygen [J]. ACS Applied Materials & Interfaces, 2021, 13(42): 49982-49992. (封面) IF=10.383,中科院2 TOP

22.     Hui Song, Zeyu Guan, Luyi Chen, Haiming Xu, Dongsheng Xia, Mingzhi Huang, Dongya Li*. Role of curvature in a carbon electronic structure under spatial confinement: conversion of nonradicals to radicals [J]. Carbon, 2021, 180: 22-30. IF=11.307,中科院1 TOP

23.     Meng Li, Dongsheng Xia, Haiming Xu, Zeyu Guan, Dongya Li*. Iron oxychloride composite sludge-derived biochar for efficient activation of peroxymonosulfate to degrade organic pollutants in wastewater [J]. Journal of Cleaner Production, 2021, 329: 129656. IF=11.072,中科院1 TOP

24.     Shiyu Zuo, Zeyu Guan, Dongsheng Xia*, Fan Yang, Haiming Xu, Mingzhi Huang, Dongya Li*. Polarized heterogeneous CuO-CN for peroxymonosulfate nonradical activation: An enhancement mechanism of mediated electron transfer[J]. Chemical Engineering Journal, 2021: 127619. IF=16.744,中科院1 TOP

25.     Hui Song, Zhuang Liu, Zeyu Guan, Fan Yang, Dongsheng Xia, Dongya Li*. Efficient persulfate non-radical activation of electron-rich copper active sites induced by oxygen on graphitic carbon nitride[J]. Science of The Total Environment, 2021, 762: 143127. IF=10.753,中科院1 TOP

26.     Shiyu Zuo, Jie Zan, Dongya Li*, Zeyu Guan, Fan Yang, Haiming Xu, Mingzhi Huang, Dongsheng Xia. Efficient Peroxymonosulfate Nonradical Activity of Zn-Mn-Al2O3@g-C3N4 via Synergism of Zn, Mn doping and g-C3N4 composite [J]. Separation and Purification Technology, 2021: 118965. IF=9.136,中科院1 TOP

27.     Shiyu Zuo, Dongsheng Xia, Zeyu Guan, Fan Yang, Binyang Zhang, Haiming Xu, Mingzhi Huang, Xuetao Guo, Dongya Li*. The Polarized Electric Field on Fe2O3/g-C3N4 for Efficient Peroxymonosulfate Activation: A Synergy of 1O2, Electron transfer and Pollutant Oxidation[J]. Separation and Purification Technology, 2021: 118717. IF=9.136,中科院1 TOP

28.     Shiyu Zuo, Dongya Li*, Fan Yang, Haiming Xu, Mingzhi Huang, Zeyu Guan*, Dongsheng Xia. Copper Oxide/Graphitic Carbon Nitride Composite for Bisphenol A Degradation by Boosted Peroxymonosulfate Activation: Mechanism of Cu-O Covalency Governs [J]. Journal of Colloid and Interface Science, 2021. IF=9.965,中科院1 TOP

29.     Zeyu Guan, Shiyu Zuo, Fan Yang, Binyang Zhang, Haiming Xu, Dongsheng Xia*, Mingzhi Huang, Dongya Li*. The p and d hybridization interaction in Fe-N-C boosts peroxymonosulfate non-radical activation[J]. Separation and Purification Technology, 2021, 258: 118025. IF=9.136,中科院1 TOP

30.     Hui Song, Zeyu Guan, Dongsheng Xia*, Haiming Xu, Fan Yang, Dongya Li*, Xiaohu Li. Copper-oxygen synergistic electronic reconstruction on g-C3N4 for efficient non-radical catalysis for peroxydisulfate and peroxymonosulfate[J]. Separation and Purification Technology, 2021, 257: 117957. IF=9.136,中科院1 TOP

31.     Shiyu Zuo, Dongsheng Xia, Zeyu Guan, Fan Yang, Shuang Cheng, Haiming Xu, Renzhuo Wan*, Dongya Li*, Min Liu. Dual-functional CuO/CN for highly efficient solar evaporation and water purification[J]. Separation and Purification Technology, 2021, 254: 117611. IF=9.136,中科院1 TOP

32.     Yi Zhu, Dongya Li*, Shiyu Zuo, Zeyu Guan, Su Ding, Dongsheng Xia, Xiaohu Li. Cu2O/CuO induced non-radical/radical pathway toward highly efficient peroxymonosulfate activation [J]. Journal of Environmental Chemical Engineering, 2021.11. IF=7.968,中科院2区)

33.     Zeyu Guan, Shiyu Zuo, Fan Yang, Binyang Zhang, Haiming Xu, Dongsheng Xia, Mingzhi Huang, Dongya Li*. The Polarized Electric Field on Fe-N-C-S Promotes Non-Radical Process of Peroxymonosulfate Degrade Diclofenac Sodium[J]. Colloids and Surfaces A: Physicochemical and Engineering Aspects, 2021: 126608. IF=5.518,中科院2区)

34.     Shiyu Zuo, Dongsheng Xia, Zeyu Guan*, Fan Yang, Jie Zan, Haiming Xu, Mingzhi Huang, Dongya Li*. Magnetite/graphite carbon nitride composite for peroxymonosulfate non-radical activation[J]. Colloids and Surfaces A: Physicochemical and Engineering Aspects, 2021, 611: 125895. IF=5.518,中科院2区)

35.     Lei Chen, Shiyu Zuo, Zeyu Guan, Haiming Xu, Dongsheng Xia*, Dongya Li*. The practical application and electron transfer mechanism of SR-Fenton activation by FeOCl [J]. Research on Chemical Intermediates, 2021, 47(2): 795-811. IF=2.26,中科院3区)

36.     Shiyu Zuo, Dongya Li*, Haiming Xu, Dongsheng Xia*. An integrated microwave-ultraviolet catalysis process of four peroxides for wastewater treatment: Free radical generation rate and mechanism[J]. Chemical Engineering Journal, 2020, 380: 122434. IF=16.744,中科院1 TOP

37.     Jie Zan, Hui Song, Shiyu Zuo, Xiangrui Chen, Dongsheng Xia*, Dongya Li*. MIL-53 (Fe)-derived Fe2O3 with oxygen vacancy as Fenton-like photocatalysts for the elimination of toxic organics in wastewater[J]. Journal of Cleaner Production, 2020, 246: 118971. IF=11.072,中科院1 TOP

38.     Weidong Hou, Haiming Xu*, Yujie Cai, Zhongwei Zou, Dongya Li*, Dongsheng Xia*. Precisely control interface OVs concentration for enhance 0D/2D Bi2O2CO3/BiOCl photocatalytic performance[J]. Applied Surface Science, 2020, 530: 147218. IF=6.18,中科院2区)

39.     Weidong Hou, Jia Yang, Haiming Xu*, Dongya Li*, Zhongwei Zou, Dongsheng Xia*. Syntheses of Nymphaea-like BiOCl with oxygen vacancies for effective removal of tetracycline hydrochloride[J]. CrystEngComm, 2020, 22(23): 3956-3964. IF=3.756,中科院3区)

40.     Binyang Zhang, Mengdie Chen, Dongya Li*, Haiming Xu, Dongsheng Xia*. Quantitative investigation into the enhancing utilization efficiency of H2O2 catalyzed by FeOCl under visible light[J]. Journal of Photochemistry and Photobiology A: Chemistry, 2020, 386: 112072. IF=3.30,中科院3区)

41.     Weidong Mei, Hui Song, Ziyi Tian, Shiyu Zuo, Dongya Li*, Haiming Xu, Dongsheng Xia*. Efficient photo-Fenton like activity in modified MIL-53 (Fe) for removal of pesticides: Regulation of photogenerated electron migration[J]. Materials Research Bulletin, 2019, 119: 110570. IF=4.02,中科院2区)

42.     Guoguan Liu, Haiming Xu*, Dongya Li*, Zhongwei Zou, Qiang Li, Dongsheng Xia*. BiOCl/BiOBr heterojunction with rich oxygen vacancies induced by ultraviolet and its enhanced photocatalytic performance[J]. European Journal of Inorganic Chemistry, 2019, 2019(46): 4887-4893. IF=2.551,中科院3区)

43.     Dongya Li, Yang Xiao, Mengjie Pu, Jie Zan, Shiyu Zuo, Haiming Xu*, Dongsheng Xia*. A metal-free protonated g-C3N4 as an effective sodium percarbonate activator at ambient pH conditions: Efficiency, stability and mechanism[J]. Materials Chemistry and Physics, 2019, 231: 225-232. IF=3.40,中科院3区)

44.     Dongya Li*, Jie Zan, Liping Wu, Shiyu Zuo, Haiming Xu*, and Dongsheng Xia*. Heterojunction tuning and catalytic efficiency of g-C3N4-Cu2O with glutamate[J]. Industrial & Engineering Chemistry Research, 2019, 58(10): 4000-4009. IF=3.57,中科院3区)

45.     Xingqi Liu, Haiming Xu*, Dongya Li*, Zhongwei Zou, Dongsheng Xia*. Facile Preparation of BiOCl/ZnO Heterostructure with Oxygen‐Rich Vacancies and Its Enhanced Photocatalytic Performance[J]. ChemistrySelect, 2019, 4(42): 12245-12251. IF=2.307,中科院4区)

46.     张斌阳,李东亚*,徐海明,孙磊,夏东升*. NaClO-PMS NaClO-O3 协同活化降解印染废水[J]. 精细化工, 2019, 5. (中文核心)

47.     Dongya Li, Shiyu Zuo, Haiming Xu*, Jie Zan, Lei Sun, Donghui Han, Wei Liao, Binyang Zhang, Dongsheng Xia*. Synthesis of a g-C3N4-Cu2O heterojunction with enhanced visible light photocatalytic activity by PEG [J]. Journal of Colloid and Interface Science, 2018, 531: 28-36. IF=9.965,中科院1 TOP

48.     Shiyu Zuo, Haiming Xu*, Wei Liao, Xiangjuan Yuan, Lei Sun, Qiang Li, Jie Zan, Dongya Li*, Dongsheng Xia*. Molten-salt synthesis of g-C3N4-Cu2O heterojunctions with highly enhanced photocatalytic performance[J]. Colloids and Surfaces A: Physicochemical and Engineering Aspects, 2018, 546: 307-315. IF=5.518,中科院2区)

49.     Jingyu Sun, Dongya Li*, Yujie Cai, Zhongwei Zou, Hua Zhang, Jiayang Gong, Lei Sun, Haiming Xu*, Dongsheng Xia*. Controllable synthesis of highly active BiOCl with different content oxygen vacancies[J]. Journal of Materials Science: Materials in Electronics, 2018, 29(14): 12241-12250. IF=2.779,中科院4区)

50.     Shiyu Zuo, Haiming Xu*, Wei Liao, Lei Sun, Donghui Han, Jie Zan, Binyang Zhang, Dongya Li*, Dongsheng Xia*. Acid‐treated g-C3N4-Cu2O composite catalyst with enhanced photocatalytic activity under visible‐light irradiation[J]. Applied Organometallic Chemistry, 2018, 32(9): e4448. IF=4.072,中科院3区)

51.     Shiyu Zuo, Haiming Xu*, Wei Liao, Lei Sun, Qiang Li, Jie Zan, Binyang Zhang, Dongya Li*, Dongsheng Xia*. Enhancement of acid treated g-C3N4-Cu2O photocatalytic activity by PEG under visible light irradiation[J]. Chemical Physics Letters, 2018, 699: 241-249. IF=2.719,中科院4区)

52.     Weidong Mei, Dongya Li*, Haiming Xu, Jie Zan, Lei Sun, Qiang Li, Binyang Zhang, Yifei Wang, Dongsheng Xia*. Effect of electronic migration of MIL-53 (Fe) on the activation of peroxymonosulfate under visible light[J]. Chemical Physics Letters, 2018, 706: 694-701. IF=2.719,中科院4区)

53.     Mengdie Chen, Haiming Xu, Qi Wang, Dongya Li*, Dongsheng Xia*. Activation mechanism of sodium percarbonate by FeOCl under visible-light-enhanced catalytic oxidation[J]. Chemical Physics Letters, 2018, 706: 415-420. IF=2.719,中科院4区)

54.     Mengdie Chen, Haiming Xu, Xiaofang Zhang, Dongya Li*, Dongsheng Xia*. Mechanism of heterogeneous activation of persulfate with FeOCl under visible light irradiation[J]. Journal of Materials Research, 2018, 33(21): 3549-3558. IF=2.909,中科院4区)

55.     Jingyu Sun, Dongya Li*, Yirui Li, Yujie Cai, Lei Sun, Xiangjuan Yuan, Gang Cao, Haiming Xu*, Dongsheng Xia*. CMC/BiOCl 3D Hierarchical Nanostructures with Exposed {001} Facets and Its Enhanced Photocatalytic Activity[J]. ChemistrySelect, 2018, 3(16): 4463-4470. IF=2.307,中科院4区)

56.     廖伟,徐海明,左诗语,肖洋,李东亚*,夏东升*. Cu2O-g-C3N4 异质结催化剂光催化降解甲基橙[J]. 化工环保, 2018 (2018 05): 552-558.(中文核心)



专利成果

以第一发明人申请国家发明专利16项,其中已授权14项。

1.       李东亚;夏东升;徐海明;袁向娟;曹刚;孙磊;陈梦蝶;王琦. [中国发明] CN201611225263.8. 利用氧基氯化铁催化活化过二硫酸盐处理有机废水的方法. (已授权)

申请日:2016-12-27 授权公告日:2019-12-24

2.       李东亚;夏东升;徐海明;袁向娟;曹刚;孙磊;陈梦蝶. [中国发明] CN201611224567.2. 利用氧基氯化铁催化活化单过硫酸盐处理有机废水的方法. (已授权)

申请日:2016-12-27 授权公告日:2019-12-24

3.       李东亚;夏东升;徐海明;袁向娟;孙磊;曹刚;陈梦蝶;王琦. [中国发明] CN201611224587.X 可见光协同FeOCl催化活化过二硫酸盐处理有机废水的方法. (已授权)

申请日:2016-12-27 授权公告日:2019-07-23

4.       李东亚;夏东升;徐海明;袁向娟;孙磊;曹刚;陈梦蝶. [中国发明] CN201611224577.6. 可见光协同FeOCl催化活化单过硫酸盐处理有机废水的方法. (已授权)

申请日:2016-12-27,授权公告日:2019-07-23

5.       李东亚;夏东升;徐海明;廖伟;左诗语;曹刚;袁向娟;孙磊[中国发明] CN201710483431.1. 一种催化过碳酸盐降解废水中有机污染物的方法. (已授权)

申请日:2017-06-22,授权公告日: 2019-10-15

6.       李东亚;夏东升;徐海明;廖伟; 左诗语;曹刚;袁向娟;孙磊;武利平[中国发明] CN201710479044.0 一种用谷氨酸改性g‑C3N4‑Cu2O复合催化剂的制备方法及其应用. (已授权)

申请日:2017-06-22,申请公告日: 2019-10-15

7.       李东亚;夏东升;徐海明;左诗语;廖伟;曹刚;袁向娟;孙磊;武利平[中国发明] CN201710479020.5. 一种用PEG改性g‑C3N4‑Cu2O复合催化剂的制备方法及其应用. (已授权)

申请日:2017-06-22,授权公告日: 2019-10-15

8.       李东亚;夏东升;徐海明;曹刚;袁向娟;孙磊;廖伟;左诗语;武利平[中国发明] CN201710479053.X.一种g‑C3N4‑Cu2O催化剂的制备方法及其应用. (已授权)

申请日:2017-06-22,授权公告日: 2019-06-25

9.       李东亚;夏东升;徐海明;左诗语;廖伟;曹刚;袁向娟;孙磊[中国发明] CN201710479009.9. 一种催化过硫酸盐降解废水中有机污染物的方法. (已授权)

申请日:2017-06-22,授权公告日: 2020-12-29

10.     李东亚;夏东升;左诗语;徐海明;孙磊 [中国发明] CN201910502983.1. 一种用于高级氧化技术的CuS-CuO-CN过氧化物复合催化剂及其制备方法和应用. (已授权)

申请日:2019-06-11,授权公告日: 2022-04-08

11.     李东亚;夏东升;左诗语;徐海明;孙磊 [中国发明] CN201910502978.0. 一种用于高级氧化技术的CuO-CN过氧化物复合催化剂及其制备方法和应用. (已授权)

申请日:2019-06-11,授权公告日: 2022-04-15

12.     李东亚;夏东升;徐海明;廖伟;左诗语;曹刚;袁向娟;孙磊[中国发明] CN201710479746.9. 一种g‑C3N4‑Cu2O复合催化剂的制备方法及其应用. (未授权)

13.     李东亚;夏东升;徐海明;袁向娟;孙磊;曹刚;廖伟;左诗语[中国发明] CN201610920449.9. 一种微波-紫外耦合催化过硫酸盐处理有机废水的方法. (未授权)

14.     李东亚;关泽宇;左诗语;丁艺琛[中国发明] CN202111316405.2. 一种硼掺杂铜氧化物催化剂及其制备方法和应用. (已授权)

申请日:2021-11-03,授权公告日: 2022-09-20

15.     李东亚;关泽宇;左诗语;朱怡 [中国发明] CN202111328686.3 一种基于金属有机配体的铜氧化物催化剂及其制备方法和应用. (未授权)

16.     李东亚;夏东升;关泽宇;李梦 [中国发明] CN202111316405.2 一种污泥基复合催化剂及其制备方法和应用. (未授权)