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成果及论文

 2024

48. F. Shi, X.Y. Li, J.Q. Di, Y.T. Xue, N. Zhang T. Y. Jin*, C.-F. Chen* and P. Chen*. Controlled Synthesis of Macrocyclic Carbazole Series with Open-Shell Polycations and Strong NIR-II-Absorbing Chiroptical Responses. CCS Chemistry, 2024, accepted.

                                                   

47. J.Q. Di, S.R. Han, P. Chen*. Recent Advances of Boron-Containing Chiral Luminescent Materials. Chin. J. Chem. 2025, 43, 219-238. (an Invited Review)

                                                                                      

46. Y. F. Shi, C. L. Li,* J. Q. Di, Y. T. Xue,  Y. W. Jia, J. X. Duan, X. Y. Hu, Y. Tian, Y. Q. Li, C. P. Sun, N. Zhang, Y. Xiong, T. Y. Jin,* and P. Chen*, Polycationic Open-Shell Cyclophanes: Synthesis of Electron-Rich Chiral Macrocycles, and Redox-Dependent Electronic States. Angew. Chem. Int. Ed. 2024, 63, e202402800.

                                       

45. X.Y. Hu, Y. Tian and P. Chen*. Unraveling Planar Chirality in Pillar[5]arenes. Tetrahedron, 2024, 162, 134088. (an Invited Review

44. Y.T. Xue, Y. F. Shi and P. Chen*.  Circularly Polarized Luminescent π-Conjugated Nanorings and Nanobelts. Adv. Optical Mater. 2024, 12, 2303322. (an Invited Review)

                                                                                          

43. 薛雨婷,孙翠萍,陈磅宽*《中国科学:化学》有机硼氮(B/N)圆偏振发光手性分子的研究进展:合成、结构及其性能表征,Sci Sin Chim, 2024, 54: 1153–1164。(手性发光专题论述

42. K. Zhang, M.Y. Hao, T. Y. Jin,  F. Shi, G.Q. Tian, C.L. Li, Y. H.W. Ma, N. Zhang, Q.S. Li,* and P. Chen*. Synthesis of π-Conjugated Chiral Aza/Boracyclophanes with a meta and para Substitution. Chem. -Eur. J. 2024, 30, e202302950. (Hot Paper)

                                                                               

2023

41. F. Zhao,# J.Y. Zhao,# H.T. Liu, Y. Wang, J.X. Duan, C.L. Li, J.Q. Di, N. Zhang, X.Y. Zheng* and P. Chen*. Synthesis of π-Conjugated Chiral Organoborane Macrocycles with Blue to Near-Infrared Emissions and the Diradical Character of Cations.  J. Am. Chem. Soc. 2023, 145, 10092-10103.

                                                   

40. C. L. Li, C. Zhang, P. F. Li, Y. W. Jia, J. X. Duan, M. Y. Liu, N. Zhang,* and P. Chen*. Red Emissive Double Aza[7]helicenes with Antiaromaticity/Aromaticity Switching via the Redox-Induced Radical Cation and Dication Species. Angew. Chem. Int. Ed. 2023, 62, e202302019.

                                                              

39. J. X. Duan, Y. F. Shi, F. Zhao, C. L. Li, Z. H. Duan, N. Zhang* and P. Chen*, Chiral Luminescent Aza[7]helicenes Functionalized with Triarylborane Acceptor and NIR-Emissive Doublet-State Radicals. Inorg. Chem. 2023, 62, 15829-15833.

                                                                                    

38. P. Li, Y.W. Jia and P. Chen*. Design and Synthesis of New Type of Macrocyclic Architectures Used for Optoelectronic Materials and Supramolecular Chemistry. Chem. -Eur. J. 2023, 29, e202300300 (an Invited Review Article) 

                                                                                                                      

37. H.J. WangY. Liu,* B.Q. YuS.Q. SongY.X. ZhengK.L LiuP. ChenH.L. WangJ.Z. JiangT.Y. Li*. A Configurationally Confined Thermally Activated Delayed Fluorescent Two-Coordinate CuI Complex for Efficient Blue Electroluminescence. Angew. Chem. Int. Ed. 2023, 62, e202217195.

36. J.F. Chen,* Q.X. Gao, L.J. Liu, P. Chen and T.B. Wei. A Pillar[5]arene-Based Planar Chiral Charge-Transfer Dye with Enhanced Circularly Polarized Luminescence and Multiple Responsive Chiroptical Changes. Chem. Sci. 2023, 14, 987-993.

2022

35. J. Song, Q. Li, P. Chen, B. Keshavarz, B. Chapman, J. Tracy, G. H. McKinley,* N. Holten-Andersen*. Dynamics of dual-junction-functionality associative polymer networks with ion and nanoparticle metal-coordinate crosslink junctions. Journal of Rheology. 2022, DOI: 10.1122/8.0000410.

34. Y. F. Shi, Y. Zeng, P. Kucheryavy, X. Yin, K. Zhang, G.Y. Meng, J. F. Chen, Q. Zhu, X.Y. Zheng*, F. Jäkle* and P. Chen*. Dynamic B/N Lewis Pairs: Insights into the Structural Variations and Photochromism via Light-Induced Fluorescence to Phosphorescence Switching. Angew. Chem. Int. Ed. 2022, 61, e202213615. Hot Paper

https://doi.org/10.1002/anie.202213615

33. Y. W. Jia, P. F. Li, K. L Liu*, C. L. Li, M. Y. Liu, J. Q. Di, N. Wang, X. Yin, N. Zhang* and P. Chen*. Expanding New Chemistry of Azabora-cyclophanes with Unique Dipolar Structures, AIE and Redox-Active Open-Shell Characteristics. Chem. Sci. 2022, 13, 11672-11679.

https://doi.org/10.1039/D2SC03581B

32. G. Q. Tian, J. F. Chen, K. Zhang, Y. F. Shi, C. L. Li, X. Yin, K. L. Liu*, and P. Chen*. Applying the B/N Lewis Pair Approach to Access Fusion-Expanded Binaphthyl-Based Chiral Analogues. Inorg. Chem. 2022, 61, 39, 15315–15319.

https://doi.org/10.1021/acs.inorgchem.2c02875


31. Y. F. Shi, C. L. Li, H. W. Ma, Z. Cao, K. L. Liu, X. Yin, N. Wang, and P. Chen*. Two-in-One Approach toward White-Light Emissions of Dimeric B/N Lewis Pairs by Tuning the Ortho-Substitution Effect. Org. Lett. 2022, 24, 29, 5497–5502.

https://pubs.acs.org/doi/10.1021/acs.orglett.2c02344


30. P. F. Li, D. Shimoyama, N. Zhang*, Y. W. Jia, G. F. Hu, C. L. Li, X. D. Yin, N. Wang, F. Jäkle* and P. ChenA New Platform of B/N-Doped Cyclophanes: Access to a p-Conjugated Block-Type B3NMacrocycle with Strong Dipole Moment and Unique Optoelectronic Properties. Angew. Chem. Int. Ed. 2022, 61e202200612. (Hot Paper

https://doi.org/10.1002/anie.202200612

29. Liu Bin, Chen Pangkuan*. Synthesis and Properties of Novel Circularly Polarized Luminescence Materials Based on Binaphthol Skeleton. Acta Chim. Sinica 2022, 80, 929-935. DOI: 10.6023/A22030122.

28. J. F. Chen, G. Q. Tian, K. L. Liu, N. Zhang, N. Wang, X.D. Yin and P. Chen. Pillar[5]arene-Based Neutral Radicals with Doublet Red Emissions and Stable Chiroptical Properties.Org. Lett. 2022, 24, 10, 1935–1940.(Featured in a Front Cover)  

https://doi.org/10.1021/acs.orglett.2c00313

      

27. F. Zhao, J.Y. Zhao, Y. Wang, H.T. Liu, N. Zhang, N. Wang, X.D. Yin, X.Y. Zheng* and P. Chen. [5]Helicene-Based Chiral Triarylboranes with Large Luminescence Dissymmetry Factor Over 10-2 Level: Synthesis and Design Strategy via Isomeric Tuning of Steric Substitutions. Dalton Transactions, 2022, 51, 6226-6234.

https://pubs.rsc.org/en/content/articlehtml/2022/dt/d2dt00677d


26. P. F. Li, Y.W. Jia, S.H. Zhang, J.Q. Di, N. Zhang and P. Chen. Oligotriarylamine-Extended Organoboranes with Tunable Electron-Donating Strength by Changing the Number of Donor Units. Inorg. Chem. 2022, 61, 9, 3951–3958.

https://doi.org/10.1021/acs.inorgchem.1c03578


25. K. Zhang, J.Y. Zhao, N. Zhang, J.F. Chen, N. Wang, X.D. Yin, X.Y. Zheng* and P. Chen. Molecular Design to Enhance Binaphthyl-Based Chiroptics Using Organoboron Chemistry in Isomeric Chiral Scaffolds. J. Mater. Chem. C. 2022, 10, 1816-1824.

https://doi.org/10.1039/D1TC05329A


24. S.H. Zhang, J.F. Chen, G.F. Hu, N. Zhang, N. Wang, X.D. Yin and P. Chen. Synthesis, Characterization, and Photophysical Properties of Triptycene-Based Chiral Organoboranes.Organometallics. 2022, 41, 99-104. (Featured in a Front Cover)

https://doi.org/10.1021/acs.organomet.1c00447

     


2021

23. C.L. Li, Y.F. Shi, P.F. Li, N. Zhang, N. Wang, X.D. Yin and P Chen. Access to Highly Luminescent N‑Doped Diazaborepins with Penta‑, Hexa‑, and Heptagon Substructures. Org. Lett. 2021, 23, 18, 7123–7128.

https://doi.org/10.1021/acs.orglett.1c02528


22. K. Zhang, G.Q. Ji, N. Zhang*, N. Wang, X.D. Yin, Q.S. Li and P Chen. Responsive Organoboranes with Dynamic Conformation of Octacyclophane-type Scaffolds: Synthesis, AIE and Temperature-dependent Dual Emissions. J. Mater. Chem. C, 2021,9, 13851-13859.

https://doi.org/10.1039/D1TC02713A


21.  J. F. Chen, X.D. Yin, K. Zhang, Z.H. Zhao, S.H. Zhang, N. Zhang, N. Wang and P Chen. Pillar[5]arene-Based Dual Chiral Organoboranes with Allowed Host−Guest Chemistry and Circularly Polarized Luminescence. J. Org. Chem. 2021, 86, 18, 12654–12663.

https://doi.org/10.1021/acs.joc.1c01175

2020

20. J. F. Chen, X. Yin, B. W. Wang, K. Zhang, G. Y. Meng, S. H. Zhang, Y. F. Shi, N. Wang, S. Wang and P. Chen. Planar Chiral Organoboranes with Thermoresponsive Emission and Circularly Polarized Luminescence: Integration of Pillar[5]arenes with Boron Chemistry. Angew. Chem. Int. Ed. 2020, 59, 11267-11272.

https://doi.org/10.1002/anie.202001145

19. G. Q. Ji, N. Wang, X. Yin and P. Chen*. Substituent Effect Induces Emission Modulation of Stilbene Photoswitches by Spatial Tuning the N/B Electronic Constraints. Org. Lett. 2020, 22, 5758-5762.

https://doi.org/10.1021/acs.orglett.0c01777


18.  P. Lei, S. Zhang, N. Zhang, X. Yin, N. Wang, and P. Chen*. Triptycene-Based Luminescent Materials in Homoconjugated Charge Transfer Systems: Synthesis, Electronic Structures, AIE Activity and Highly Tunable Emissions. ACS Omega, 2020, 5, 28606-28614.

https://doi.org/10.1021/acsomega.0c03565

2019

17.  J. F. Chen, G. Y. Meng, Q. Zhu, S. H. Zhang, P. Chen*. Pillar[5]arenes: a New Class of AIEgen Macrocycles Used for Luminescence Sensing of Fe3+ Ion. J. Mater. Chem. C. 2019, 7, 11747-11751.

https://doi.org/10.1039/C9TC03831K


16.  Q. Zhu, S. Wang and P. Chen*. Diazocine Derivatives: A Family of Azobenzenes for Photochromism with Highly Enhanced Turn-On Fluorescence. Org. Lett. 2019, 21, 4025-4029.

https://doi.org/10.1021/acs.orglett.9b01215


15. J. F. Chen, P. Chen*. Pillar[5]arene-Based Resilient Supramolecular Gel with Dual-Stimuli Responses and Self-Healing Properties. ACS Appl. Polym. Mater. 2019, 1, 2224-2229.

https://doi.org/10.1021/acsapm.9b00516


14. C.J. Sun, N. Wang, T. Peng, X. Yin, S. Wang, and P. Chen. BN Functionalized Benzotrithiophene-Based Azaborines: Synthesis, Structures and Anion Binding Properties.Inorg. Chem. 2019, 58, 3591-3595.

https://doi.org/10.1021/acs.inorgchem.8b03579


2018

13. Y. Shi, S. K. Mellerup, K. Yuan, G. Hu, F. Sauriol, T. Peng, N. Wang*, P. Chen*, S. Wang*. Stabilising fleeting intermediates of stilbene photocyclization with amino-borane functionalization: the rare isolation of persistent dihydrophenanthrenes and their [1,5]H-shift isomers. Chem. Sci. 2018, 9, 3844-3855.

https://doi.org/10.1039/C8SC00560E


12. Q.G. Hou, L.J. Liu, S.K. Mellerup, N. Wang, T. Peng, P. Chen, and S. Wang. Stimuli-responsive B/N Lewis Pairs Based on the Modulation of B-N Bond Strength. Org. Lett. 2018, 20, 6467-6470.

https://doi.org/10.1021/acs.orglett.8b02774



2016年以前代表性文章

11. P. Chen, Q. Li, S. Grindy, and N. Holten-Andersen. White-Light-Emitting Lanthanide Metallogels with Tunable Luminescence and Reversible Stimuli-Responsive Properties. J. Am. Chem. Soc. 2015, 137, 11590-11593(Highly Cited Paper; Highlighted by C&E News)

https://doi.org/10.1021/jacs.5b07394

10. P. Chen, X. Yin, N. Baser-Kirazli and F. Jäkle. Versatile Design Principles for Facile Access to Unstrained Conjugated Organoborane Macrocycles.  Angew. Chem. Int. Ed. 2015, 54, 10768-10772.

https://doi.org/10.1002/anie.201503219


9. P. Chen, R. A. Lalancette, and F. Jäkle. π–Expanded Borazines: An Ambipolar Conjugated B–π–N Macrocyle. Angew. Chem. Int. Ed. 2012, 51, 7994-7998. (Highlighted by C&E News)

https://doi.org/10.1002/anie.201203788

8. P. Chen, and F. Jäkle. Highly Luminescent Electron-Deficient Bora-cyclophanes. J. Am. Chem. Soc. 2011, 133, 20142-20145. (Highlighted by C&E News; JACS Spotlights; JACS Selects; VIP ; Angewandte Highlights

https://doi.org/10.1021/ja209602z

7. P. Chen, R. A. Lalancette, and F. Jäkle. Applying the Oligomer Approach to Luminescent Conjugated Organoboranes. J. Am. Chem. Soc. 2011, 133, 8802-8805.

https://doi.org/10.1021/ja201436a


6. P. Chen,# A. S. Marshall,# S.H. Chi, X. Yin, J. W. Perry, and F. Jäkle. Luminescent Quadrupolar Borazine Oligomers: Synthesis, Photophysics and Two-Photon Absorption Properties. Chem.-Eur. J. 2015, 21, 18237-18247.

5. P. Chen, and N. Holten-Andersen. Multistimuli-Responsive White Luminescent Fluids Using Hybrid Lanthanide Metal-Coordinate Complex Probes. Adv. Opt. Mater. 2015, 3, 1041-1046.

4. P. Chen, Y. Qi, Y.X. Che, and J. Zheng. Network topology and property studies for two binodal self-penetrated coordination polymers. CrystEngComm. 2010, 12, 720-724.

3. P. Chen, S. R. Batten, Y. Qi, and J. Zheng, Two 3-D cluster-based frameworks: Highly eight-connected molecular topology and magnetism. Cryst. Growth & Des. 2009, 9, 2756-2761.

2. P. Chen, Y.X. Che, J. Zheng, and S. R. Batten. Heteronuclear Metamagnet Showing Spin Canting and Single-Crystal to Single-Crystal Phase Transformation. Chem. Mater. 2007, 19, 2162-2167.

1. P. Chen, L. Xue, J. Zheng. Two 2-Fold Interpenetrated Frameworks Showing Different Topologies Based on the Isomerous Benzenedi-carboxylate Mixed with a Flexible N, N’-Type Ligand. Cryst. Growth & Des. 2006, 6, 2517-2522.