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成果及论文

 Before Fudan U.

29.    C. Zhu+,* J. Liu+, B. K. Mai, F. Himo,* J.-E. Bäckvall*, Efficient Stereoselective Carbocyclization to cis-1,4-Disubstituted Heterocycles Enabled by Dual Pd/Electron Transfer Mediator (ETM) Catalysis. J. Am. Chem. Soc. 2020, 142, 5751-5759.

28.    C. Zhu+,* J. Liu+, M.-b. Li+, J.-E. Bäckvall*, Palladium-catalyzed oxidative dehydrogenative carbonylation reactions using carbon monoxide and mechanistic overviews. Chem. Soc. Rev. 2020, 49, 341-353.

27.    M.-B. Li, D. Posevins, A. Geoffroy, C. Zhu,* J.-E. Bäckvall*, Efficient Heterogeneous Palladium-Catalyzed Oxidative Cascade Reactions of Enallenols to Furan and Oxaborole Derivatives. Angew. Chem. Int. Ed. 2020, 59, 1992-1996.

26.    C. Zhu*, J.-E. Bäckvall*, An Efficient Approach to Regio- and Stereodefined Fully-Substituted Alkenylsilanes by Pd-Catalyzed Allenic C(sp3)-H Oxidation. Chem. Eur. J. 2019, 25, 11566-11573.

25.    C. Zhu+,* B. Yang+, B. K. Mai, S. Palazzotto, Y. Qiu, A. Gudmundsson, A. Ricke, F. Himo,* J.-E. Bäckvall*, Highly Selective Palladium-Catalyzed Hydroborylative Carbocyclization of Bisallenes to Seven-Membered Rings, J. Am. Chem. Soc. 2018, 140,  14324-14333.

24.    C. Zhu, J. L. Schwarz, S. Cembellín, S. Greßies, F. Glorius*, Highly Selective Manganese(I)/Lewis Acid Cocatalyzed Direct C‒H Propargylation Using Bromoallenes, Angew. Chem. Int. Ed. 2018, 57, 437-441.

23.    C. Zhu+, T. Pinkert+, S. Greßies, F. Glorius*, One-Pot C–H Formylation Enabled by Relay Catalysis of Manganese(I) and Iron(III), ACS Catal. 2018, 8, 10036-10042.

22.    B. Yang, Y. Qiu, T. Jiang, W. D. Wulff, X. Yin, C. Zhu,* J.-E. Bäckvall*, Enantioselective Pd-Catalyzed Carbonylative Carbocyclization of Enallenes via Cross-Dehydrogenative Coupling with Terminal Alkynes: Efficient Construction of α-Chirality of Ketones, Angew. Chem. Int. Ed. 2017, 56, 4535-4539.

21.    Y. Qiu, B. Yang, T. Jiang, C. Zhu, J.-E. Bäckvall*, Palladium-Catalyzed Oxidative Cascade Carbonylative Spirolactonization of Enallenols, Angew. Chem. Int. Ed. 2017, 56, 3221-3225.

20.    Y. Qiu, B. Yang, C. Zhu, J.-E. Bäckvall*, Highly Selective Olefin-Assisted  Palladium-Catalyzed Oxidative Carbocyclization via Remote Olefin Insertion, Chem. Sci. 2017, 8, 616-620.

19.    C. Zhu+,* B. Yang+, Y. Qiu, J.-E. Bäckvall*, Highly Selective Construction of Seven-Membered Carbocycles by Olefin-Assisted Palladium-Catalyzed Oxidative Carbocyclization–Alkoxycarbonylation of Bisallenes, Angew. Chem. Int. Ed. 2016, 55, 14405-14408.

18.    Y. Qiu, B. Yang, C. Zhu,* J.-E. Bäckvall*, Palladium-Catalyzed Oxidative Carbocyclization-Borylation of Enallenes to Cyclobutenes, Angew. Chem. Int. Ed. 2016, 55, 6520-6524.

17.    B. Yang+, C. Zhu+, Y. Qiu, J.-E. Bäckvall*, Enzyme- and Ruthenium-Catalyzed Enantioselective Transformation of α-Allenic Alcohols to 2,3-Dihydrofurans, Angew. Chem. Int. Ed. 2016, 55, 5568-5572.

16.    C. Zhu+, B. Yang+, Y. Qiu, J.-E. Bäckvall*, Olefin-Directed Palladium-Catalyzed Regio-and Stereoselective Hydroborationof Allenes, Chem. Eur. J. 2016, 22, 2939-2943.

15.    Y. Qiu, B.  Yang, C. Zhu, J. E. Bäckvall*, Highly Efficient Cascade Reaction for Selective Formation of Spirocyclobutenes from Dienallenes via Palladium-Catalyzed Oxidative Double Carbocyclization-Carbonylation-Alkynylation, J. Am. Chem. Soc. 2016, 138, 13846-13849.

14.    T. Jiang, X. Quan, C. Zhu, P. G. Andersson, J.-E. Bäckvall*, Palladium-Catalyzed Oxidative Synthesis of α-Acetoxylated Enones from Alkynes, Angew. Chem. Int. Ed. 2016, 55, 5824-5828.

13.    C. Zhu, B. Yang, J.-E. Bäckvall*, Highly Selective Cascade C-C Bond Formation via Palladium-Catalyzed Oxidative Carbonylation-Carbocyclization-Carbonylation-Alkynylation of Enallenes, J. Am. Chem. Soc. 2015, 137, 11868-11871.

12.    C. Zhu, B. Yang, T. Jiang, J.-E. Bäckvall*, Olefin-Directed Palladium-Catalyzed Regio-and Stereoselective Oxidative Arylation of Allenes, Angew. Chem. Int. Ed. 2015, 54, 9066-9069.

11.    C. Zhu, S. Ma*, Sc(OTf)3-Catalyzed Bicyclization of o-Alkynylanilines with Aldehydes: Ring-Fused 1,2-Dihydroquinolines, Angew. Chem. Int. Ed. 2014, 53, 13532-13535.

10.    C. Zhu, S. Ma*, Efficient Carbazole Synthesis via Pd/Cu-Cocatalyzed Cross-Coupling/Isomerization of 2-Allyl-3-iodoindoles and Terminalalkynes, Org. Lett. 2014, 16, 1542-1545.

9.        B. Chen+, C. Zhu+, Y. Tang, S. Ma*, Copper-mediated pyrazole synthesis from 2,3-allenoates or 2-alkynoates, amines and nitriles, Chem. Commun.2014, 50, 7677-7679.

8.        C. Zhu, S. Ma*, Studies on Palladium-Catalyzed Efficient Synthesis of Dihydrocycloocta[b]indoles and Their Thermal Reactivities with Maleimide or Maleic Anhydride, Adv. Synth. Catal. 2014, 356, 3897-3911.

7.        W. Lin, T. Cao, W. Fan, Y. Han, J. Kuang, H. Luo, B. Miao, X. Tang, Q. Yu, W. Yuan, J. Zhang, C. Zhu, S. Ma*, Enantioselective Double Manipulation on Tetrahydroisoquinolines with Terminal Alkynes and Aldehydes under Cu(I) Catalysis, Angew. Chem. Int. Ed. 2014, 53, 277-281.

6.        C. Zhu, S. Ma*, Coupling and Cyclization of o-Iodoanilines and Propargylic Bromides via Allenes: An Efficient Entry to Indomethacin, Org. Lett. 2013, 15, 2782-2785.

5.        X. Tang, C. Zhu, T. Cao, J. Kuang, W. Lin, S. Ni, J. Zhang, S. Ma*, Cadmium iodide-mediated allenylation of alkynes with ketones, Nature Commun. 2013, 4, 2450.

4.        S. Ni, C. Zhu, J. Chen, S. Ma*, Preparation of 1-Benzyl-2-methyl-3- (ethoxycarbonyl)-4-(2-phenylethyl)-1H-pyrrole from 4-Phenyl-1,2-butadiene, Org. Synth. 2013, 90, 327-337.

3.        R. Lü, J. Ye, T. Cao, B. Chen, W. Fan, W. Lin, J. Liu, H. Luo, B. Miao, S. Ni, X. Tang, N. Wang, Y. Wang, X. Xie, Q. Yu, W. Yuan, W. Zhang, C. Zhu, S. Ma*, Bimetallic Enantioselective Approach to Axially Chiral Allenes, Org. Lett. 2013, 15, 2254-2257.

2.        C. Zhu, X. Zhang, X. Lian, S. Ma*, One-Pot Approach to Installing Eight-Membered Rings onto Indoles, Angew. Chem. Int. Ed. 2012, 51, 7817-7820.

1.        J. Cheng, X. Jiang, C. Zhu, S. Ma*, Palladium-Catalyzed Three-Component Tandem Cyclization Reaction of 2-(2,3-Allenyl)acylacetates, Organic Halides, and Amines: An Effective Protocol for the Synthesis of 4,5-Dihydro-1H-pyrrole Derivatives, Adv. Synth. Catal. 2011, 353, 1676-1682.

       (+equal contribution,; *corresponding author)