Constructing Defective Heterojunctions of BiOBr Nanosheets and Hollow NH2-functionalized MOFs for Visible-light-driven CO2 Reduction with Nearly 100% CO Selectivity by Pure H2O,Chemistry - An Asian Journal

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Constructing Defective Heterojunctions of BiOBr Nanosheets and Hollow NH2-functionalized MOFs for Visible-light-driven CO2 Reduction with Nearly 100% CO Selectivity by Pure H2O
Chemistry - An Asian Journal ( IF 3.5 ) Pub Date : 2023-02-12 , DOI: 10.1002/asia.202300033
Menghan Yang ₁ , Yali Han ₁ , Junfang Ding ₁ , Yan Guo ₁ , Chenhui Han ₁ , Xiaojun Gu ₁

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BiOBr nanoplates were successfully attached to hollow NH₂-MIL-125(Ti) surface to form Z-format defect heterojunction. In pure water, the optimized oxygen-containing vacancy catalyst reduced CO₂ to CO with near 100% selective high-efficiency visible light, and the rate of CO formation reached 459.7 μmol g⁻¹ h⁻¹, which is higher than that of all photocatalysts reported previously.

中文翻译：

构建 BiOBr 纳米片和中空 NH2 功能化 MOF 的缺陷异质结，用于可见光驱动的 CO2 还原，纯 H2O 对 CO 的选择性接近 100%

BiOBr 纳米片成功附着在空心NH ₂ -MIL-125(Ti) 表面形成Z 型缺陷异质结。在纯水中，优化的含氧空位催化剂将CO ₂还原为CO，选择性接近100%的高效可见光，CO生成速率达到459.7 μmol g ⁻¹ h ⁻¹，高于所有催化剂先前报道的光催化剂。

更新日期：2023-02-12

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