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Heterogenization of Salen Metal Molecular Catalysts in Covalent Organic Frameworks for Photocatalytic Hydrogen Evolution
Angewandte Chemie International Edition ( IF 16.1 ) Pub Date : 2022-11-19 , DOI: 10.1002/anie.202214143 Wei Zhou 1 , Qi-Wen Deng 1 , Hui-Jie He 1 , Li Yang 1 , Tian-Yi Liu 1 , Xiao Wang 1 , Dao-Yuan Zheng 1 , Zhang-Ben Dai 2 , Lei Sun 1 , Chengcheng Liu 1 , Hao Wu 1 , Zhen Li 1 , Wei-Qiao Deng 1
Angewandte Chemie International Edition ( IF 16.1 ) Pub Date : 2022-11-19 , DOI: 10.1002/anie.202214143 Wei Zhou 1 , Qi-Wen Deng 1 , Hui-Jie He 1 , Li Yang 1 , Tian-Yi Liu 1 , Xiao Wang 1 , Dao-Yuan Zheng 1 , Zhang-Ben Dai 2 , Lei Sun 1 , Chengcheng Liu 1 , Hao Wu 1 , Zhen Li 1 , Wei-Qiao Deng 1
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The heterogenization of a Salen metal complex molecular catalyst into a rigid covalent organic framework (COF) through covalent linkage with the light-harvesting unit of pyrene for photocatalytic hydrogen evolution is reported. Co/Zn-Salen-COF showed the best hydrogen evolution activity (1378 μmol g−1 h−1), which is superior to the previously reported non-noble metal-based COF photocatalysts
中文翻译：
用于光催化析氢的共价有机骨架中 Salen 金属分子催化剂的异质化
报道了通过与芘的光捕获单元共价连接，将 Salen 金属配合物分子催化剂异质化为刚性共价有机骨架 (COF)，用于光催化析氢。Co/Zn-Salen-COF表现出最佳的析氢活性（1378 μmol g −1 h −1），优于之前报道的非贵金属基COF光催化剂
更新日期：2022-11-19
中文翻译：
用于光催化析氢的共价有机骨架中 Salen 金属分子催化剂的异质化
报道了通过与芘的光捕获单元共价连接，将 Salen 金属配合物分子催化剂异质化为刚性共价有机骨架 (COF)，用于光催化析氢。Co/Zn-Salen-COF表现出最佳的析氢活性（1378 μmol g −1 h −1），优于之前报道的非贵金属基COF光催化剂
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