Porous Organic Polymers for Post‐Combustion Carbon Capture,Advanced Materials

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Porous Organic Polymers for Post‐Combustion Carbon Capture
Advanced Materials ( IF 27.4 ) Pub Date : 2017-07-25 , DOI: 10.1002/adma.201700229
Lanfang Zou ₁ , Yujia Sun ₁ , Sai Che ₁ , Xinyu Yang ₁ , Xuan Wang ₁ , Mathieu Bosch ₁ , Qi Wang ₁ , Hao Li ₁ , Mallory Smith ₁ , Shuai Yuan ₁ , Zachary Perry ₁ , Hong‐Cai Zhou _{1,

2}

Affiliation

One of the most pressing environmental concerns of our age is the escalating level of atmospheric CO₂. Intensive efforts have been made to investigate advanced porous materials, especially porous organic polymers (POPs), as one type of the most promising candidates for carbon capture due to their extremely high porosity, structural diversity, and physicochemical stability. This review provides a critical and in‐depth analysis of recent POP research as it pertains to carbon capture. The definitions and terminologies commonly used to evaluate the performance of POPs for carbon capture, including CO₂ capacity, enthalpy, selectivity, and regeneration strategies, are summarized. A detailed correlation study between the structural and chemical features of POPs and their adsorption capacities is discussed, mainly focusing on the physical interactions and chemical reactions. Finally, a concise outlook for utilizing POPs for carbon capture is discussed, noting areas in which further work is needed to develop the next‐generation POPs for practical applications.

中文翻译：

燃烧后碳捕获的多孔有机聚合物

当今时代最紧迫的环境问题之一是大气中CO _2的水平不断上升。由于其极高的孔隙率，结构多样性和物理化学稳定性，人们已经为研究先进的多孔材料，特别是多孔有机聚合物（POP）进行了深入的研究，作为碳捕获的最有希望的候选者之一。这篇综述提供了与碳捕集有关的最新持久性有机污染物研究的重要而深入的分析。通常用于评估POPs碳捕获（包括CO _2）性能的定义和术语总结了容量，焓，选择性和再生策略。讨论了持久性有机污染物的结构和化学特征与其吸附能力之间的详细相关性研究，主要侧重于物理相互作用和化学反应。最后，讨论了利用POPs进行碳捕集的简明前景，并指出了需要进一步开展工作以开发用于实际应用的下一代POPs的领域。

更新日期：2017-07-25

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